Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2

Photocatalytic water splitting on TiO2 is a promising route to H2 fuel production, but the mechanistic pathway at the water–TiO2 interface remains poorly understood. Here, using liquid environmental TEM and first-principles calculations, the authors unveil the formation of a self-hydrogenated shell...

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Autores principales:	Yue Lu, Wen-Jin Yin, Kai-Lin Peng, Kuan Wang, Qi Hu, Annabella Selloni, Fu-Rong Chen, Li-Min Liu, Man-Ling Sui
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2018
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/4764dc8bd72e496d907de40748535713
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spelling	oai:doaj.org-article:4764dc8bd72e496d907de407485357132021-12-02T16:49:21ZSelf-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO210.1038/s41467-018-05144-12041-1723https://doaj.org/article/4764dc8bd72e496d907de407485357132018-07-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05144-1https://doaj.org/toc/2041-1723Photocatalytic water splitting on TiO2 is a promising route to H2 fuel production, but the mechanistic pathway at the water–TiO2 interface remains poorly understood. Here, using liquid environmental TEM and first-principles calculations, the authors unveil the formation of a self-hydrogenated shell on the TiO2 surface that further promotes H2 production.Yue LuWen-Jin YinKai-Lin PengKuan WangQi HuAnnabella SelloniFu-Rong ChenLi-Min LiuMan-Ling SuiNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-9 (2018)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Yue Lu Wen-Jin Yin Kai-Lin Peng Kuan Wang Qi Hu Annabella Selloni Fu-Rong Chen Li-Min Liu Man-Ling Sui Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2
description	Photocatalytic water splitting on TiO2 is a promising route to H2 fuel production, but the mechanistic pathway at the water–TiO2 interface remains poorly understood. Here, using liquid environmental TEM and first-principles calculations, the authors unveil the formation of a self-hydrogenated shell on the TiO2 surface that further promotes H2 production.
format	article
author	Yue Lu Wen-Jin Yin Kai-Lin Peng Kuan Wang Qi Hu Annabella Selloni Fu-Rong Chen Li-Min Liu Man-Ling Sui
author_facet	Yue Lu Wen-Jin Yin Kai-Lin Peng Kuan Wang Qi Hu Annabella Selloni Fu-Rong Chen Li-Min Liu Man-Ling Sui
author_sort	Yue Lu
title	Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2
title_short	Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2
title_full	Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2
title_fullStr	Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2
title_full_unstemmed	Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2
title_sort	self-hydrogenated shell promoting photocatalytic h2 evolution on anatase tio2
publisher	Nature Portfolio
publishDate	2018
url	https://doaj.org/article/4764dc8bd72e496d907de40748535713
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Self-hydrogenated shell promoting photocatalytic H2 evolution on anatase TiO2

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