Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon

Efficient electroreduction of CO2 to multi-carbon products is challenging. Here, the single atom Cu encapsulated on N-doped porous carbon catalysts are designed for reducing CO2 to acetone at low overpotentials and the active sites are identified as Cu coordination with four pyrrole-N atoms.

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Autores principales: Kun Zhao, Xiaowa Nie, Haozhi Wang, Shuo Chen, Xie Quan, Hongtao Yu, Wonyong Choi, Guanghui Zhang, Bupmo Kim, Jingguang G. Chen
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/49018fcfd4784022ab1870ec15ebd6c4
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Sumario:Efficient electroreduction of CO2 to multi-carbon products is challenging. Here, the single atom Cu encapsulated on N-doped porous carbon catalysts are designed for reducing CO2 to acetone at low overpotentials and the active sites are identified as Cu coordination with four pyrrole-N atoms.