Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon

Efficient electroreduction of CO2 to multi-carbon products is challenging. Here, the single atom Cu encapsulated on N-doped porous carbon catalysts are designed for reducing CO2 to acetone at low overpotentials and the active sites are identified as Cu coordination with four pyrrole-N atoms.

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Autores principales: Kun Zhao, Xiaowa Nie, Haozhi Wang, Shuo Chen, Xie Quan, Hongtao Yu, Wonyong Choi, Guanghui Zhang, Bupmo Kim, Jingguang G. Chen
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/49018fcfd4784022ab1870ec15ebd6c4
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spelling oai:doaj.org-article:49018fcfd4784022ab1870ec15ebd6c42021-12-02T15:54:44ZSelective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon10.1038/s41467-020-16381-82041-1723https://doaj.org/article/49018fcfd4784022ab1870ec15ebd6c42020-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-16381-8https://doaj.org/toc/2041-1723Efficient electroreduction of CO2 to multi-carbon products is challenging. Here, the single atom Cu encapsulated on N-doped porous carbon catalysts are designed for reducing CO2 to acetone at low overpotentials and the active sites are identified as Cu coordination with four pyrrole-N atoms.Kun ZhaoXiaowa NieHaozhi WangShuo ChenXie QuanHongtao YuWonyong ChoiGuanghui ZhangBupmo KimJingguang G. ChenNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-10 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Kun Zhao
Xiaowa Nie
Haozhi Wang
Shuo Chen
Xie Quan
Hongtao Yu
Wonyong Choi
Guanghui Zhang
Bupmo Kim
Jingguang G. Chen
Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon
description Efficient electroreduction of CO2 to multi-carbon products is challenging. Here, the single atom Cu encapsulated on N-doped porous carbon catalysts are designed for reducing CO2 to acetone at low overpotentials and the active sites are identified as Cu coordination with four pyrrole-N atoms.
format article
author Kun Zhao
Xiaowa Nie
Haozhi Wang
Shuo Chen
Xie Quan
Hongtao Yu
Wonyong Choi
Guanghui Zhang
Bupmo Kim
Jingguang G. Chen
author_facet Kun Zhao
Xiaowa Nie
Haozhi Wang
Shuo Chen
Xie Quan
Hongtao Yu
Wonyong Choi
Guanghui Zhang
Bupmo Kim
Jingguang G. Chen
author_sort Kun Zhao
title Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon
title_short Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon
title_full Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon
title_fullStr Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon
title_full_unstemmed Selective electroreduction of CO2 to acetone by single copper atoms anchored on N-doped porous carbon
title_sort selective electroreduction of co2 to acetone by single copper atoms anchored on n-doped porous carbon
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/49018fcfd4784022ab1870ec15ebd6c4
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AT guanghuizhang selectiveelectroreductionofco2toacetonebysinglecopperatomsanchoredonndopedporouscarbon
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