Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction

A systematic time-resolved study can provide key insights on selective carbon dioxide electro-reduction. Here, the authors report operando seconds-resolved X-ray absorption spectroscopy to uncover the chemical state evolution of working catalysts in a carbon dioxide electroreduction process.

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Autores principales: Sheng-Chih Lin, Chun-Chih Chang, Shih-Yun Chiu, Hsiao-Tien Pai, Tzu-Yu Liao, Chia-Shuo Hsu, Wei-Hung Chiang, Ming-Kang Tsai, Hao Ming Chen
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Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/492699f113f14fd98afccda780fc8ccb
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spelling oai:doaj.org-article:492699f113f14fd98afccda780fc8ccb2021-12-02T18:36:59ZOperando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction10.1038/s41467-020-17231-32041-1723https://doaj.org/article/492699f113f14fd98afccda780fc8ccb2020-07-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-17231-3https://doaj.org/toc/2041-1723A systematic time-resolved study can provide key insights on selective carbon dioxide electro-reduction. Here, the authors report operando seconds-resolved X-ray absorption spectroscopy to uncover the chemical state evolution of working catalysts in a carbon dioxide electroreduction process.Sheng-Chih LinChun-Chih ChangShih-Yun ChiuHsiao-Tien PaiTzu-Yu LiaoChia-Shuo HsuWei-Hung ChiangMing-Kang TsaiHao Ming ChenNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-12 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Sheng-Chih Lin
Chun-Chih Chang
Shih-Yun Chiu
Hsiao-Tien Pai
Tzu-Yu Liao
Chia-Shuo Hsu
Wei-Hung Chiang
Ming-Kang Tsai
Hao Ming Chen
Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction
description A systematic time-resolved study can provide key insights on selective carbon dioxide electro-reduction. Here, the authors report operando seconds-resolved X-ray absorption spectroscopy to uncover the chemical state evolution of working catalysts in a carbon dioxide electroreduction process.
format article
author Sheng-Chih Lin
Chun-Chih Chang
Shih-Yun Chiu
Hsiao-Tien Pai
Tzu-Yu Liao
Chia-Shuo Hsu
Wei-Hung Chiang
Ming-Kang Tsai
Hao Ming Chen
author_facet Sheng-Chih Lin
Chun-Chih Chang
Shih-Yun Chiu
Hsiao-Tien Pai
Tzu-Yu Liao
Chia-Shuo Hsu
Wei-Hung Chiang
Ming-Kang Tsai
Hao Ming Chen
author_sort Sheng-Chih Lin
title Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction
title_short Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction
title_full Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction
title_fullStr Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction
title_full_unstemmed Operando time-resolved X-ray absorption spectroscopy reveals the chemical nature enabling highly selective CO2 reduction
title_sort operando time-resolved x-ray absorption spectroscopy reveals the chemical nature enabling highly selective co2 reduction
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/492699f113f14fd98afccda780fc8ccb
work_keys_str_mv AT shengchihlin operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT chunchihchang operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT shihyunchiu operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT hsiaotienpai operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT tzuyuliao operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT chiashuohsu operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT weihungchiang operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT mingkangtsai operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
AT haomingchen operandotimeresolvedxrayabsorptionspectroscopyrevealsthechemicalnatureenablinghighlyselectiveco2reduction
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