Molecular alignment in degenerated dissociation channels in strong laser fields

Abstract In this work, we study strong-field molecular alignment in, for the first time, degenerated channels following the same charged states of molecules. By measuring the angular distribution of dissociation fragments from two degenerated N+ + N+ channels of N2, we observe an opposite angular di...

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Autores principales: Wei Lai, Alan Heins, Chunlei Guo
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Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/4986b7bdea2b46d183fc2265d8770cc9
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spelling oai:doaj.org-article:4986b7bdea2b46d183fc2265d8770cc92021-12-02T15:05:43ZMolecular alignment in degenerated dissociation channels in strong laser fields10.1038/s41598-017-02738-52045-2322https://doaj.org/article/4986b7bdea2b46d183fc2265d8770cc92017-05-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-02738-5https://doaj.org/toc/2045-2322Abstract In this work, we study strong-field molecular alignment in, for the first time, degenerated channels following the same charged states of molecules. By measuring the angular distribution of dissociation fragments from two degenerated N+ + N+ channels of N2, we observe an opposite angular distribution development in these two channels, one expanding and one contracting, when the laser intensity increases. Our further study shows that the expanding channel comes from a nonsequential transition, while the contracting channel involves a sequential transition. We also study the time sequence of the sequential and nonsequential transitions and find that the opposite angular distribution development is due to the different degrees of molecular alignment in these two degenerated channels.Wei LaiAlan HeinsChunlei GuoNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-7 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Wei Lai
Alan Heins
Chunlei Guo
Molecular alignment in degenerated dissociation channels in strong laser fields
description Abstract In this work, we study strong-field molecular alignment in, for the first time, degenerated channels following the same charged states of molecules. By measuring the angular distribution of dissociation fragments from two degenerated N+ + N+ channels of N2, we observe an opposite angular distribution development in these two channels, one expanding and one contracting, when the laser intensity increases. Our further study shows that the expanding channel comes from a nonsequential transition, while the contracting channel involves a sequential transition. We also study the time sequence of the sequential and nonsequential transitions and find that the opposite angular distribution development is due to the different degrees of molecular alignment in these two degenerated channels.
format article
author Wei Lai
Alan Heins
Chunlei Guo
author_facet Wei Lai
Alan Heins
Chunlei Guo
author_sort Wei Lai
title Molecular alignment in degenerated dissociation channels in strong laser fields
title_short Molecular alignment in degenerated dissociation channels in strong laser fields
title_full Molecular alignment in degenerated dissociation channels in strong laser fields
title_fullStr Molecular alignment in degenerated dissociation channels in strong laser fields
title_full_unstemmed Molecular alignment in degenerated dissociation channels in strong laser fields
title_sort molecular alignment in degenerated dissociation channels in strong laser fields
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/4986b7bdea2b46d183fc2265d8770cc9
work_keys_str_mv AT weilai molecularalignmentindegenerateddissociationchannelsinstronglaserfields
AT alanheins molecularalignmentindegenerateddissociationchannelsinstronglaserfields
AT chunleiguo molecularalignmentindegenerateddissociationchannelsinstronglaserfields
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