Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids

The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and contact forces, which are both key to nonlinear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flo...

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Autores principales: Taiki Yanagishima, Yanyan Liu, Hajime Tanaka, Roel P. A. Dullens
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Lenguaje:EN
Publicado: American Physical Society 2021
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Acceso en línea:https://doaj.org/article/4b3ead862f66464bb1e4d512f992f47f
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spelling oai:doaj.org-article:4b3ead862f66464bb1e4d512f992f47f2021-12-02T14:58:42ZParticle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids10.1103/PhysRevX.11.0210562160-3308https://doaj.org/article/4b3ead862f66464bb1e4d512f992f47f2021-06-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.11.021056http://doi.org/10.1103/PhysRevX.11.021056https://doaj.org/toc/2160-3308The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and contact forces, which are both key to nonlinear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flow. To fully elucidate the role of rotational dynamics experimentally, it is crucial to measure the translational and rotational motion of all spheres simultaneously. Here, we directly access hydrodynamic and frictional coupling in colloidal suspensions up to arbitrarily high volume fractions using compositionally uniform colloidal spheres with an off-center, fully embedded core. We reveal interparticle hydrodynamic rotation-rotation coupling in charged colloidal crystals. We also find that higher local crystallinity in denser hard-sphere crystalline sediments enhances rotational diffusivity and that nearly arrested particles exhibit a stick-slip rotational motion due to frictional coupling. Our findings shed new light on the largely unexplored, local rotational dynamics of spherical particles in dense particulate materials.Taiki YanagishimaYanyan LiuHajime TanakaRoel P. A. DullensAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 11, Iss 2, p 021056 (2021)
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
spellingShingle Physics
QC1-999
Taiki Yanagishima
Yanyan Liu
Hajime Tanaka
Roel P. A. Dullens
Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
description The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and contact forces, which are both key to nonlinear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flow. To fully elucidate the role of rotational dynamics experimentally, it is crucial to measure the translational and rotational motion of all spheres simultaneously. Here, we directly access hydrodynamic and frictional coupling in colloidal suspensions up to arbitrarily high volume fractions using compositionally uniform colloidal spheres with an off-center, fully embedded core. We reveal interparticle hydrodynamic rotation-rotation coupling in charged colloidal crystals. We also find that higher local crystallinity in denser hard-sphere crystalline sediments enhances rotational diffusivity and that nearly arrested particles exhibit a stick-slip rotational motion due to frictional coupling. Our findings shed new light on the largely unexplored, local rotational dynamics of spherical particles in dense particulate materials.
format article
author Taiki Yanagishima
Yanyan Liu
Hajime Tanaka
Roel P. A. Dullens
author_facet Taiki Yanagishima
Yanyan Liu
Hajime Tanaka
Roel P. A. Dullens
author_sort Taiki Yanagishima
title Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
title_short Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
title_full Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
title_fullStr Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
title_full_unstemmed Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
title_sort particle-level visualization of hydrodynamic and frictional couplings in dense suspensions of spherical colloids
publisher American Physical Society
publishDate 2021
url https://doaj.org/article/4b3ead862f66464bb1e4d512f992f47f
work_keys_str_mv AT taikiyanagishima particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids
AT yanyanliu particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids
AT hajimetanaka particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids
AT roelpadullens particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids
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