Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids
The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and contact forces, which are both key to nonlinear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flo...
Guardado en:
Autores principales: | , , , |
---|---|
Formato: | article |
Lenguaje: | EN |
Publicado: |
American Physical Society
2021
|
Materias: | |
Acceso en línea: | https://doaj.org/article/4b3ead862f66464bb1e4d512f992f47f |
Etiquetas: |
Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
|
id |
oai:doaj.org-article:4b3ead862f66464bb1e4d512f992f47f |
---|---|
record_format |
dspace |
spelling |
oai:doaj.org-article:4b3ead862f66464bb1e4d512f992f47f2021-12-02T14:58:42ZParticle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids10.1103/PhysRevX.11.0210562160-3308https://doaj.org/article/4b3ead862f66464bb1e4d512f992f47f2021-06-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.11.021056http://doi.org/10.1103/PhysRevX.11.021056https://doaj.org/toc/2160-3308The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and contact forces, which are both key to nonlinear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flow. To fully elucidate the role of rotational dynamics experimentally, it is crucial to measure the translational and rotational motion of all spheres simultaneously. Here, we directly access hydrodynamic and frictional coupling in colloidal suspensions up to arbitrarily high volume fractions using compositionally uniform colloidal spheres with an off-center, fully embedded core. We reveal interparticle hydrodynamic rotation-rotation coupling in charged colloidal crystals. We also find that higher local crystallinity in denser hard-sphere crystalline sediments enhances rotational diffusivity and that nearly arrested particles exhibit a stick-slip rotational motion due to frictional coupling. Our findings shed new light on the largely unexplored, local rotational dynamics of spherical particles in dense particulate materials.Taiki YanagishimaYanyan LiuHajime TanakaRoel P. A. DullensAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 11, Iss 2, p 021056 (2021) |
institution |
DOAJ |
collection |
DOAJ |
language |
EN |
topic |
Physics QC1-999 |
spellingShingle |
Physics QC1-999 Taiki Yanagishima Yanyan Liu Hajime Tanaka Roel P. A. Dullens Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids |
description |
The rotational Brownian motion of colloidal spheres in dense suspensions reflects local hydrodynamics and contact forces, which are both key to nonlinear rheological phenomena such as shear-thickening and jamming, and transport in crowded environments, including intracellular migration and blood flow. To fully elucidate the role of rotational dynamics experimentally, it is crucial to measure the translational and rotational motion of all spheres simultaneously. Here, we directly access hydrodynamic and frictional coupling in colloidal suspensions up to arbitrarily high volume fractions using compositionally uniform colloidal spheres with an off-center, fully embedded core. We reveal interparticle hydrodynamic rotation-rotation coupling in charged colloidal crystals. We also find that higher local crystallinity in denser hard-sphere crystalline sediments enhances rotational diffusivity and that nearly arrested particles exhibit a stick-slip rotational motion due to frictional coupling. Our findings shed new light on the largely unexplored, local rotational dynamics of spherical particles in dense particulate materials. |
format |
article |
author |
Taiki Yanagishima Yanyan Liu Hajime Tanaka Roel P. A. Dullens |
author_facet |
Taiki Yanagishima Yanyan Liu Hajime Tanaka Roel P. A. Dullens |
author_sort |
Taiki Yanagishima |
title |
Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids |
title_short |
Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids |
title_full |
Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids |
title_fullStr |
Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids |
title_full_unstemmed |
Particle-Level Visualization of Hydrodynamic and Frictional Couplings in Dense Suspensions of Spherical Colloids |
title_sort |
particle-level visualization of hydrodynamic and frictional couplings in dense suspensions of spherical colloids |
publisher |
American Physical Society |
publishDate |
2021 |
url |
https://doaj.org/article/4b3ead862f66464bb1e4d512f992f47f |
work_keys_str_mv |
AT taikiyanagishima particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids AT yanyanliu particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids AT hajimetanaka particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids AT roelpadullens particlelevelvisualizationofhydrodynamicandfrictionalcouplingsindensesuspensionsofsphericalcolloids |
_version_ |
1718389262596964352 |