Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation

Identifying active sites and designing rationally heterogeneous catalysts are not inherently straightforward due to their complexity. Here, the authors reveal the nature of active sites for efficient C–H bond activation in C1-C4 alkanes over bare ZrO2 and provide fundamentals for controlling their c...

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Autores principales:	Yaoyuan Zhang, Yun Zhao, Tatiana Otroshchenko, Henrik Lund, Marga-Martina Pohl, Uwe Rodemerck, David Linke, Haijun Jiao, Guiyuan Jiang, Evgenii V. Kondratenko
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2018
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/4c744b4417544b0cbdd0cba437b9cbf6
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spelling	oai:doaj.org-article:4c744b4417544b0cbdd0cba437b9cbf62021-12-02T15:34:07ZControl of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation10.1038/s41467-018-06174-52041-1723https://doaj.org/article/4c744b4417544b0cbdd0cba437b9cbf62018-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-06174-5https://doaj.org/toc/2041-1723Identifying active sites and designing rationally heterogeneous catalysts are not inherently straightforward due to their complexity. Here, the authors reveal the nature of active sites for efficient C–H bond activation in C1-C4 alkanes over bare ZrO2 and provide fundamentals for controlling their concentration.Yaoyuan ZhangYun ZhaoTatiana OtroshchenkoHenrik LundMarga-Martina PohlUwe RodemerckDavid LinkeHaijun JiaoGuiyuan JiangEvgenii V. KondratenkoNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-10 (2018)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Yaoyuan Zhang Yun Zhao Tatiana Otroshchenko Henrik Lund Marga-Martina Pohl Uwe Rodemerck David Linke Haijun Jiao Guiyuan Jiang Evgenii V. Kondratenko Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation
description	Identifying active sites and designing rationally heterogeneous catalysts are not inherently straightforward due to their complexity. Here, the authors reveal the nature of active sites for efficient C–H bond activation in C1-C4 alkanes over bare ZrO2 and provide fundamentals for controlling their concentration.
format	article
author	Yaoyuan Zhang Yun Zhao Tatiana Otroshchenko Henrik Lund Marga-Martina Pohl Uwe Rodemerck David Linke Haijun Jiao Guiyuan Jiang Evgenii V. Kondratenko
author_facet	Yaoyuan Zhang Yun Zhao Tatiana Otroshchenko Henrik Lund Marga-Martina Pohl Uwe Rodemerck David Linke Haijun Jiao Guiyuan Jiang Evgenii V. Kondratenko
author_sort	Yaoyuan Zhang
title	Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation
title_short	Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation
title_full	Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation
title_fullStr	Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation
title_full_unstemmed	Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation
title_sort	control of coordinatively unsaturated zr sites in zro2 for efficient c–h bond activation
publisher	Nature Portfolio
publishDate	2018
url	https://doaj.org/article/4c744b4417544b0cbdd0cba437b9cbf6
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_version_	1718386897374412800

Control of coordinatively unsaturated Zr sites in ZrO2 for efficient C–H bond activation

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