Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
Abstract A method to determine the doping induced charge carrier profiles in lightly and moderately doped organic semiconductor thin films is presented. The theory of the method of Charge Extraction by a Linearly Increasing Voltage technique in the doping-induced capacitive regime (doping-CELIV) is...
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Nature Portfolio
2017
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oai:doaj.org-article:4c95e62705734f06b84b7903a40de3162021-12-02T15:05:57ZDoping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients10.1038/s41598-017-05499-32045-2322https://doaj.org/article/4c95e62705734f06b84b7903a40de3162017-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-05499-3https://doaj.org/toc/2045-2322Abstract A method to determine the doping induced charge carrier profiles in lightly and moderately doped organic semiconductor thin films is presented. The theory of the method of Charge Extraction by a Linearly Increasing Voltage technique in the doping-induced capacitive regime (doping-CELIV) is extended to the case with non-uniform doping profiles and the analytical description is verified with drift-diffusion simulations. The method is demonstrated experimentally on evaporated organic small-molecule thin films with a controlled doping profile, and solution-processed thin films where the non-uniform doping profile is unintentional, probably induced during the deposition process, and a priori unknown. Furthermore, the method offers a possibility of directly probing charge-density distributions at interfaces between highly doped and lightly doped or undoped layers.Mathias NymanOskar J. SandbergStaffan DahlströmDonato SpoltoreChristian KörnerYadong ZhangStephen BarlowSeth R. MarderKarl LeoKoen VandewalRonald ÖsterbackaNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017) |
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Medicine R Science Q Mathias Nyman Oskar J. Sandberg Staffan Dahlström Donato Spoltore Christian Körner Yadong Zhang Stephen Barlow Seth R. Marder Karl Leo Koen Vandewal Ronald Österbacka Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
description |
Abstract A method to determine the doping induced charge carrier profiles in lightly and moderately doped organic semiconductor thin films is presented. The theory of the method of Charge Extraction by a Linearly Increasing Voltage technique in the doping-induced capacitive regime (doping-CELIV) is extended to the case with non-uniform doping profiles and the analytical description is verified with drift-diffusion simulations. The method is demonstrated experimentally on evaporated organic small-molecule thin films with a controlled doping profile, and solution-processed thin films where the non-uniform doping profile is unintentional, probably induced during the deposition process, and a priori unknown. Furthermore, the method offers a possibility of directly probing charge-density distributions at interfaces between highly doped and lightly doped or undoped layers. |
format |
article |
author |
Mathias Nyman Oskar J. Sandberg Staffan Dahlström Donato Spoltore Christian Körner Yadong Zhang Stephen Barlow Seth R. Marder Karl Leo Koen Vandewal Ronald Österbacka |
author_facet |
Mathias Nyman Oskar J. Sandberg Staffan Dahlström Donato Spoltore Christian Körner Yadong Zhang Stephen Barlow Seth R. Marder Karl Leo Koen Vandewal Ronald Österbacka |
author_sort |
Mathias Nyman |
title |
Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
title_short |
Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
title_full |
Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
title_fullStr |
Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
title_full_unstemmed |
Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
title_sort |
doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/4c95e62705734f06b84b7903a40de316 |
work_keys_str_mv |
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1718388642026618880 |