Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients

Abstract A method to determine the doping induced charge carrier profiles in lightly and moderately doped organic semiconductor thin films is presented. The theory of the method of Charge Extraction by a Linearly Increasing Voltage technique in the doping-induced capacitive regime (doping-CELIV) is...

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Autores principales: Mathias Nyman, Oskar J. Sandberg, Staffan Dahlström, Donato Spoltore, Christian Körner, Yadong Zhang, Stephen Barlow, Seth R. Marder, Karl Leo, Koen Vandewal, Ronald Österbacka
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/4c95e62705734f06b84b7903a40de316
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spelling oai:doaj.org-article:4c95e62705734f06b84b7903a40de3162021-12-02T15:05:57ZDoping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients10.1038/s41598-017-05499-32045-2322https://doaj.org/article/4c95e62705734f06b84b7903a40de3162017-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-05499-3https://doaj.org/toc/2045-2322Abstract A method to determine the doping induced charge carrier profiles in lightly and moderately doped organic semiconductor thin films is presented. The theory of the method of Charge Extraction by a Linearly Increasing Voltage technique in the doping-induced capacitive regime (doping-CELIV) is extended to the case with non-uniform doping profiles and the analytical description is verified with drift-diffusion simulations. The method is demonstrated experimentally on evaporated organic small-molecule thin films with a controlled doping profile, and solution-processed thin films where the non-uniform doping profile is unintentional, probably induced during the deposition process, and a priori unknown. Furthermore, the method offers a possibility of directly probing charge-density distributions at interfaces between highly doped and lightly doped or undoped layers.Mathias NymanOskar J. SandbergStaffan DahlströmDonato SpoltoreChristian KörnerYadong ZhangStephen BarlowSeth R. MarderKarl LeoKoen VandewalRonald ÖsterbackaNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Mathias Nyman
Oskar J. Sandberg
Staffan Dahlström
Donato Spoltore
Christian Körner
Yadong Zhang
Stephen Barlow
Seth R. Marder
Karl Leo
Koen Vandewal
Ronald Österbacka
Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
description Abstract A method to determine the doping induced charge carrier profiles in lightly and moderately doped organic semiconductor thin films is presented. The theory of the method of Charge Extraction by a Linearly Increasing Voltage technique in the doping-induced capacitive regime (doping-CELIV) is extended to the case with non-uniform doping profiles and the analytical description is verified with drift-diffusion simulations. The method is demonstrated experimentally on evaporated organic small-molecule thin films with a controlled doping profile, and solution-processed thin films where the non-uniform doping profile is unintentional, probably induced during the deposition process, and a priori unknown. Furthermore, the method offers a possibility of directly probing charge-density distributions at interfaces between highly doped and lightly doped or undoped layers.
format article
author Mathias Nyman
Oskar J. Sandberg
Staffan Dahlström
Donato Spoltore
Christian Körner
Yadong Zhang
Stephen Barlow
Seth R. Marder
Karl Leo
Koen Vandewal
Ronald Österbacka
author_facet Mathias Nyman
Oskar J. Sandberg
Staffan Dahlström
Donato Spoltore
Christian Körner
Yadong Zhang
Stephen Barlow
Seth R. Marder
Karl Leo
Koen Vandewal
Ronald Österbacka
author_sort Mathias Nyman
title Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
title_short Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
title_full Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
title_fullStr Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
title_full_unstemmed Doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
title_sort doping-induced carrier profiles in organic semiconductors determined from capacitive extraction-current transients
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/4c95e62705734f06b84b7903a40de316
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