Confinement suppresses instabilities in particle-laden droplets

Abstract Tiny concentrations of suspended particles may alter the behavior of an evaporating droplet remarkably, leading to partially viscous and partially elastic dynamical characteristics. This, in turn, may lead to some striking mechanical instabilities, such as buckling and rupture. Here, we rep...

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Autores principales: Lalit Bansal, Saptarshi Basu, Suman Chakraborty
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/5196ae07da0d460e968d65846dd80037
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spelling oai:doaj.org-article:5196ae07da0d460e968d65846dd800372021-12-02T12:32:37ZConfinement suppresses instabilities in particle-laden droplets10.1038/s41598-017-08126-32045-2322https://doaj.org/article/5196ae07da0d460e968d65846dd800372017-08-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-08126-3https://doaj.org/toc/2045-2322Abstract Tiny concentrations of suspended particles may alter the behavior of an evaporating droplet remarkably, leading to partially viscous and partially elastic dynamical characteristics. This, in turn, may lead to some striking mechanical instabilities, such as buckling and rupture. Here, we report certain non-trivial implications of the consequent morpho-dynamics (macro to nano scales), when such an evaporating droplet is encapsulated in a confined environment. Compared to unconfined scenario, we report non-intuitive suppression of rupturing beyond a critical confinement. We attribute this to confinement-induced dramatic alteration in the evaporating flux, leading to distinctive spatio-temporal characteristics of the internal flow leading to preferential particle transport and subsequent morphological transitions. We present a regime map quantifying buckling-non buckling pathways. These results may turn out to be of profound importance towards achieving desired morphological features of a colloidal droplet, by aptly tuning the confinement space, initial particle concentration, as well as the initial droplet volume.Lalit BansalSaptarshi BasuSuman ChakrabortyNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-8 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Lalit Bansal
Saptarshi Basu
Suman Chakraborty
Confinement suppresses instabilities in particle-laden droplets
description Abstract Tiny concentrations of suspended particles may alter the behavior of an evaporating droplet remarkably, leading to partially viscous and partially elastic dynamical characteristics. This, in turn, may lead to some striking mechanical instabilities, such as buckling and rupture. Here, we report certain non-trivial implications of the consequent morpho-dynamics (macro to nano scales), when such an evaporating droplet is encapsulated in a confined environment. Compared to unconfined scenario, we report non-intuitive suppression of rupturing beyond a critical confinement. We attribute this to confinement-induced dramatic alteration in the evaporating flux, leading to distinctive spatio-temporal characteristics of the internal flow leading to preferential particle transport and subsequent morphological transitions. We present a regime map quantifying buckling-non buckling pathways. These results may turn out to be of profound importance towards achieving desired morphological features of a colloidal droplet, by aptly tuning the confinement space, initial particle concentration, as well as the initial droplet volume.
format article
author Lalit Bansal
Saptarshi Basu
Suman Chakraborty
author_facet Lalit Bansal
Saptarshi Basu
Suman Chakraborty
author_sort Lalit Bansal
title Confinement suppresses instabilities in particle-laden droplets
title_short Confinement suppresses instabilities in particle-laden droplets
title_full Confinement suppresses instabilities in particle-laden droplets
title_fullStr Confinement suppresses instabilities in particle-laden droplets
title_full_unstemmed Confinement suppresses instabilities in particle-laden droplets
title_sort confinement suppresses instabilities in particle-laden droplets
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/5196ae07da0d460e968d65846dd80037
work_keys_str_mv AT lalitbansal confinementsuppressesinstabilitiesinparticleladendroplets
AT saptarshibasu confinementsuppressesinstabilitiesinparticleladendroplets
AT sumanchakraborty confinementsuppressesinstabilitiesinparticleladendroplets
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