The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts

The active sites over oxide-derived copper (OD-Cu) catalysts for CO2 electroreduction are unclear. Here, the authors show atom-level product-specific active sites on OD-Cu surface models, where planar and convex square sites are responsible for ethylene while the step square site favours alcohols ge...

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Autores principales: Dongfang Cheng, Zhi-Jian Zhao, Gong Zhang, Piaoping Yang, Lulu Li, Hui Gao, Sihang Liu, Xin Chang, Sai Chen, Tuo Wang, Geoffrey A. Ozin, Zhipan Liu, Jinlong Gong
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Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/525e59fc8e934fed895670142e971e2c
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spelling oai:doaj.org-article:525e59fc8e934fed895670142e971e2c2021-12-02T14:11:51ZThe nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts10.1038/s41467-020-20615-02041-1723https://doaj.org/article/525e59fc8e934fed895670142e971e2c2021-01-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-20615-0https://doaj.org/toc/2041-1723The active sites over oxide-derived copper (OD-Cu) catalysts for CO2 electroreduction are unclear. Here, the authors show atom-level product-specific active sites on OD-Cu surface models, where planar and convex square sites are responsible for ethylene while the step square site favours alcohols generation.Dongfang ChengZhi-Jian ZhaoGong ZhangPiaoping YangLulu LiHui GaoSihang LiuXin ChangSai ChenTuo WangGeoffrey A. OzinZhipan LiuJinlong GongNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-8 (2021)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Dongfang Cheng
Zhi-Jian Zhao
Gong Zhang
Piaoping Yang
Lulu Li
Hui Gao
Sihang Liu
Xin Chang
Sai Chen
Tuo Wang
Geoffrey A. Ozin
Zhipan Liu
Jinlong Gong
The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
description The active sites over oxide-derived copper (OD-Cu) catalysts for CO2 electroreduction are unclear. Here, the authors show atom-level product-specific active sites on OD-Cu surface models, where planar and convex square sites are responsible for ethylene while the step square site favours alcohols generation.
format article
author Dongfang Cheng
Zhi-Jian Zhao
Gong Zhang
Piaoping Yang
Lulu Li
Hui Gao
Sihang Liu
Xin Chang
Sai Chen
Tuo Wang
Geoffrey A. Ozin
Zhipan Liu
Jinlong Gong
author_facet Dongfang Cheng
Zhi-Jian Zhao
Gong Zhang
Piaoping Yang
Lulu Li
Hui Gao
Sihang Liu
Xin Chang
Sai Chen
Tuo Wang
Geoffrey A. Ozin
Zhipan Liu
Jinlong Gong
author_sort Dongfang Cheng
title The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
title_short The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
title_full The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
title_fullStr The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
title_full_unstemmed The nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
title_sort nature of active sites for carbon dioxide electroreduction over oxide-derived copper catalysts
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/525e59fc8e934fed895670142e971e2c
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