Oxidation States, Thouless’ Pumps, and Nontrivial Ionic Transport in Nonstoichiometric Electrolytes

Thouless’ quantization of adiabatic particle transport permits one to associate an integer topological charge with each atom of an electronically gapped material. If these charges are additive and independent of atomic positions, they provide a rigorous definition of atomic oxidation states and atom...

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Autores principales: Paolo Pegolo, Federico Grasselli, Stefano Baroni
Formato: article
Lenguaje:EN
Publicado: American Physical Society 2020
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Acceso en línea:https://doaj.org/article/533cbe27d79445eba8eef881f1ec5861
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