Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions

In this study, a magnetic iron-zirconium modified zeolite (FeZrMZ) was synthesized. Through sediment culture experiments, the influence of the addition of modified materials on the migration and transformation of phosphorus in river sediments was investigated. The results showed that the modified ze...

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Autores principales: Chunlei Wang, Herong Gui, Chen Li, Jiayu Chen, Chen Chen
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Publicado: IWA Publishing 2021
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spelling oai:doaj.org-article:569bb11be7f44c7e856f1d84bf8515222021-11-06T11:18:26ZEffect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions0273-12231996-973210.2166/wst.2021.271https://doaj.org/article/569bb11be7f44c7e856f1d84bf8515222021-08-01T00:00:00Zhttp://wst.iwaponline.com/content/84/4/941https://doaj.org/toc/0273-1223https://doaj.org/toc/1996-9732In this study, a magnetic iron-zirconium modified zeolite (FeZrMZ) was synthesized. Through sediment culture experiments, the influence of the addition of modified materials on the migration and transformation of phosphorus in river sediments was investigated. The results showed that the modified zeolite could not only effectively reduce the phosphorus concentration in the overlying water, but also significantly reduce the phosphorus concentration in the pore water of sediments. The addition of modified zeolite makes the unstable weakly adsorbed phosphorus (NH4Cl-P) and redox phosphorus (BD-P) transform into the more stable metal oxide-bound phosphorus (NaOH-P) and very stable residual phosphorus (Res-P). The four types of bioavailable phosphorus (BAP), including water-soluble phosphorus (WSP), readily desorbable phosphorus (RDP), algae-available phosphorus (AAP), and NaHCO3 extractable phosphorus (Olsen-P). Under anoxic conditions, they were reduced by 53.5%, 14.1%, 23.8%, and 49.9% respectively. Under aerobic conditions, they were reduced by 23.2%, 16.6%, 32.1%, and 50.0%. The addition of magnetic iron-zirconium modified zeolite could clearly reduce the release potential of phosphorus in sediment, and it could be recovered through the action of an external magnetic field, so it could be used as an effective sediment modifier to control the sediment release of phosphorus. HIGHLIGHTS Synthesize and characterize FeZrMZ, which has a good magnetic separation ability.; FeZrMZ can effectively reduce the concentration of phosphorus in overlying water and interstitial water.; FeZrMZ can convert unstable phosphorus in sediments into stable phosphorus.;Chunlei WangHerong GuiChen LiJiayu ChenChen ChenIWA Publishingarticlemagnetic iron-zirconium modified zeolitemost variable p formsphosphorus migrationsedimentEnvironmental technology. Sanitary engineeringTD1-1066ENWater Science and Technology, Vol 84, Iss 4, Pp 941-953 (2021)
institution DOAJ
collection DOAJ
language EN
topic magnetic iron-zirconium modified zeolite
most variable p forms
phosphorus migration
sediment
Environmental technology. Sanitary engineering
TD1-1066
spellingShingle magnetic iron-zirconium modified zeolite
most variable p forms
phosphorus migration
sediment
Environmental technology. Sanitary engineering
TD1-1066
Chunlei Wang
Herong Gui
Chen Li
Jiayu Chen
Chen Chen
Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
description In this study, a magnetic iron-zirconium modified zeolite (FeZrMZ) was synthesized. Through sediment culture experiments, the influence of the addition of modified materials on the migration and transformation of phosphorus in river sediments was investigated. The results showed that the modified zeolite could not only effectively reduce the phosphorus concentration in the overlying water, but also significantly reduce the phosphorus concentration in the pore water of sediments. The addition of modified zeolite makes the unstable weakly adsorbed phosphorus (NH4Cl-P) and redox phosphorus (BD-P) transform into the more stable metal oxide-bound phosphorus (NaOH-P) and very stable residual phosphorus (Res-P). The four types of bioavailable phosphorus (BAP), including water-soluble phosphorus (WSP), readily desorbable phosphorus (RDP), algae-available phosphorus (AAP), and NaHCO3 extractable phosphorus (Olsen-P). Under anoxic conditions, they were reduced by 53.5%, 14.1%, 23.8%, and 49.9% respectively. Under aerobic conditions, they were reduced by 23.2%, 16.6%, 32.1%, and 50.0%. The addition of magnetic iron-zirconium modified zeolite could clearly reduce the release potential of phosphorus in sediment, and it could be recovered through the action of an external magnetic field, so it could be used as an effective sediment modifier to control the sediment release of phosphorus. HIGHLIGHTS Synthesize and characterize FeZrMZ, which has a good magnetic separation ability.; FeZrMZ can effectively reduce the concentration of phosphorus in overlying water and interstitial water.; FeZrMZ can convert unstable phosphorus in sediments into stable phosphorus.;
format article
author Chunlei Wang
Herong Gui
Chen Li
Jiayu Chen
Chen Chen
author_facet Chunlei Wang
Herong Gui
Chen Li
Jiayu Chen
Chen Chen
author_sort Chunlei Wang
title Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
title_short Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
title_full Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
title_fullStr Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
title_full_unstemmed Effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
title_sort effect of magnetic iron-zirconium modified zeolite on the different phosphorus forms in river sediment under aerobic and anoxic conditions
publisher IWA Publishing
publishDate 2021
url https://doaj.org/article/569bb11be7f44c7e856f1d84bf851522
work_keys_str_mv AT chunleiwang effectofmagneticironzirconiummodifiedzeoliteonthedifferentphosphorusformsinriversedimentunderaerobicandanoxicconditions
AT heronggui effectofmagneticironzirconiummodifiedzeoliteonthedifferentphosphorusformsinriversedimentunderaerobicandanoxicconditions
AT chenli effectofmagneticironzirconiummodifiedzeoliteonthedifferentphosphorusformsinriversedimentunderaerobicandanoxicconditions
AT jiayuchen effectofmagneticironzirconiummodifiedzeoliteonthedifferentphosphorusformsinriversedimentunderaerobicandanoxicconditions
AT chenchen effectofmagneticironzirconiummodifiedzeoliteonthedifferentphosphorusformsinriversedimentunderaerobicandanoxicconditions
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