Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring
<p>Vertical profiles of the mass concentration of black carbon (BC) were measured at altitudes up to 5 km during the PAMARCMiP (Polar Airborne Measurements and Arctic Regional Climate Model simulation Project) aircraft-based field experiment conducted around the northern Greenland Sea (Fram St...
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Copernicus Publications
2021
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Physics QC1-999 Chemistry QD1-999 S. Ohata S. Ohata M. Koike A. Yoshida A. Yoshida N. Moteki K. Adachi N. Oshima H. Matsui O. Eppers O. Eppers H. Bozem M. Zanatta M. Zanatta A. B. Herber Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring |
| description |
<p>Vertical profiles of the mass concentration of black carbon (BC) were
measured at altitudes up to 5 km during the PAMARCMiP (Polar Airborne Measurements and Arctic Regional Climate Model simulation Project) aircraft-based field
experiment conducted around the northern Greenland Sea (Fram Strait) during
March and April 2018 from operation base Station Nord (81.6<span class="inline-formula"><sup>∘</sup></span> N,
16.7<span class="inline-formula"><sup>∘</sup></span> W). Median BC mass concentrations in individual altitude
ranges were 7–18 ng m<span class="inline-formula"><sup>−3</sup></span> at standard temperature and pressure at
altitudes below 4.5 km. These concentrations were systematically lower than
previous observations in the Arctic in spring, conducted by ARCTAS-A in 2008
and NETCARE in 2015, and similar to those observed during HIPPO3 in 2010.
Column amounts of BC for altitudes below 5 km in the Arctic (<span class="inline-formula"><i>></i>66.5</span><span class="inline-formula"><sup>∘</sup></span> N; COL<span class="inline-formula"><sub>BC</sub></span>), observed during the ARCTAS-A and NETCARE
experiments, were higher by factors of 4.2 and 2.7, respectively, than those
of the PAMARCMiP experiment. These differences could not be explained solely
by the different locations of the experiments. The year-to-year variation of
COL<span class="inline-formula"><sub>BC</sub></span> values generally corresponded to that of biomass burning activities
in northern midlatitudes over western and eastern Eurasia. Furthermore,
numerical model simulations estimated the year-to-year variation of
contributions from anthropogenic sources to be smaller than 30 %–40 %.
These results suggest that the year-to-year variation of biomass burning
activities likely affected BC amounts in the Arctic troposphere in spring,
at least in the years examined in this study. The year-to-year variations in
BC mass concentrations were also observed at the surface at high Arctic
sites Ny-Ålesund and Utqiaġvik (formerly known as Barrow, the location of
Barrow Atmospheric Baseline Observatory), although their magnitudes were slightly
lower than those in COL<span class="inline-formula"><sub>BC</sub></span>.</p>
<p>Numerical model simulations in general successfully reproduced the observed
COL<span class="inline-formula"><sub>BC</sub></span> values for PAMARCMiP and HIPPO3 (within a factor of 2), whereas they
markedly underestimated the values for ARCTAS-A and NETCARE by factors of
3.7–5.8 and 3.3–5.0, respectively. Because anthropogenic contributions
account for nearly all of the COL<span class="inline-formula"><sub>BC</sub></span> (82 %–98 %) in PAMARCMiP and HIPPO3,
the good agreement between the observations and calculations for these two
experiments suggests that anthropogenic contributions were<span id="page15862"/> generally well
reproduced. However, the significant underestimations of COL<span class="inline-formula"><sub>BC</sub></span> for
ARCTAS-A and NETCARE suggest that biomass burning contributions were
underestimated. In this study, we also investigated plumes with enhanced BC
mass concentrations, which were affected by biomass burning emissions,
observed at 5 km altitude. Interestingly, the mass-averaged diameter of BC
(core) and the shell-to-core diameter ratio of BC-containing particles in
the plumes were generally not very different from those in other air
samples, which were considered to be mostly aged anthropogenic BC. These
observations provide a useful basis to evaluate numerical model simulations of
the BC radiative effect in the Arctic region in spring.</p> |
| format |
article |
| author |
S. Ohata S. Ohata M. Koike A. Yoshida A. Yoshida N. Moteki K. Adachi N. Oshima H. Matsui O. Eppers O. Eppers H. Bozem M. Zanatta M. Zanatta A. B. Herber |
| author_facet |
S. Ohata S. Ohata M. Koike A. Yoshida A. Yoshida N. Moteki K. Adachi N. Oshima H. Matsui O. Eppers O. Eppers H. Bozem M. Zanatta M. Zanatta A. B. Herber |
| author_sort |
S. Ohata |
| title |
Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring |
| title_short |
Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring |
| title_full |
Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring |
| title_fullStr |
Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring |
| title_full_unstemmed |
Arctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring |
| title_sort |
arctic black carbon during pamarcmip 2018 and previous aircraft experiments in spring |
| publisher |
Copernicus Publications |
| publishDate |
2021 |
| url |
https://doaj.org/article/584071f0dc7c47f7b658ae8698f1fb96 |
| work_keys_str_mv |
AT sohata arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT sohata arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT mkoike arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT ayoshida arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT ayoshida arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT nmoteki arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT kadachi arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT noshima arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT hmatsui arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT oeppers arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT oeppers arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT hbozem arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT mzanatta arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT mzanatta arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring AT abherber arcticblackcarbonduringpamarcmip2018andpreviousaircraftexperimentsinspring |
| _version_ |
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| spelling |
oai:doaj.org-article:584071f0dc7c47f7b658ae8698f1fb962021-11-04T08:00:11ZArctic black carbon during PAMARCMiP 2018 and previous aircraft experiments in spring10.5194/acp-21-15861-20211680-73161680-7324https://doaj.org/article/584071f0dc7c47f7b658ae8698f1fb962021-11-01T00:00:00Zhttps://acp.copernicus.org/articles/21/15861/2021/acp-21-15861-2021.pdfhttps://doaj.org/toc/1680-7316https://doaj.org/toc/1680-7324<p>Vertical profiles of the mass concentration of black carbon (BC) were measured at altitudes up to 5 km during the PAMARCMiP (Polar Airborne Measurements and Arctic Regional Climate Model simulation Project) aircraft-based field experiment conducted around the northern Greenland Sea (Fram Strait) during March and April 2018 from operation base Station Nord (81.6<span class="inline-formula"><sup>∘</sup></span> N, 16.7<span class="inline-formula"><sup>∘</sup></span> W). Median BC mass concentrations in individual altitude ranges were 7–18 ng m<span class="inline-formula"><sup>−3</sup></span> at standard temperature and pressure at altitudes below 4.5 km. These concentrations were systematically lower than previous observations in the Arctic in spring, conducted by ARCTAS-A in 2008 and NETCARE in 2015, and similar to those observed during HIPPO3 in 2010. Column amounts of BC for altitudes below 5 km in the Arctic (<span class="inline-formula"><i>></i>66.5</span><span class="inline-formula"><sup>∘</sup></span> N; COL<span class="inline-formula"><sub>BC</sub></span>), observed during the ARCTAS-A and NETCARE experiments, were higher by factors of 4.2 and 2.7, respectively, than those of the PAMARCMiP experiment. These differences could not be explained solely by the different locations of the experiments. The year-to-year variation of COL<span class="inline-formula"><sub>BC</sub></span> values generally corresponded to that of biomass burning activities in northern midlatitudes over western and eastern Eurasia. Furthermore, numerical model simulations estimated the year-to-year variation of contributions from anthropogenic sources to be smaller than 30 %–40 %. These results suggest that the year-to-year variation of biomass burning activities likely affected BC amounts in the Arctic troposphere in spring, at least in the years examined in this study. The year-to-year variations in BC mass concentrations were also observed at the surface at high Arctic sites Ny-Ålesund and Utqiaġvik (formerly known as Barrow, the location of Barrow Atmospheric Baseline Observatory), although their magnitudes were slightly lower than those in COL<span class="inline-formula"><sub>BC</sub></span>.</p> <p>Numerical model simulations in general successfully reproduced the observed COL<span class="inline-formula"><sub>BC</sub></span> values for PAMARCMiP and HIPPO3 (within a factor of 2), whereas they markedly underestimated the values for ARCTAS-A and NETCARE by factors of 3.7–5.8 and 3.3–5.0, respectively. Because anthropogenic contributions account for nearly all of the COL<span class="inline-formula"><sub>BC</sub></span> (82 %–98 %) in PAMARCMiP and HIPPO3, the good agreement between the observations and calculations for these two experiments suggests that anthropogenic contributions were<span id="page15862"/> generally well reproduced. However, the significant underestimations of COL<span class="inline-formula"><sub>BC</sub></span> for ARCTAS-A and NETCARE suggest that biomass burning contributions were underestimated. In this study, we also investigated plumes with enhanced BC mass concentrations, which were affected by biomass burning emissions, observed at 5 km altitude. Interestingly, the mass-averaged diameter of BC (core) and the shell-to-core diameter ratio of BC-containing particles in the plumes were generally not very different from those in other air samples, which were considered to be mostly aged anthropogenic BC. These observations provide a useful basis to evaluate numerical model simulations of the BC radiative effect in the Arctic region in spring.</p>S. OhataS. OhataM. KoikeA. YoshidaA. YoshidaN. MotekiK. AdachiN. OshimaH. MatsuiO. EppersO. EppersH. BozemM. ZanattaM. ZanattaA. B. HerberCopernicus PublicationsarticlePhysicsQC1-999ChemistryQD1-999ENAtmospheric Chemistry and Physics, Vol 21, Pp 15861-15881 (2021) |