d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery

Low intrinsic activity and accessibility of active sites limit the application of metal-organic framework as catalyst for Zn-air battery. Here, authors present a cation substitution strategy to regulate the electronic state of metal sites and modify its porosity, which enables battery operation.

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Autores principales:	Yi Jiang, Ya-Ping Deng, Ruilin Liang, Jing Fu, Rui Gao, Dan Luo, Zhengyu Bai, Yongfeng Hu, Aiping Yu, Zhongwei Chen
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2020
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/5d710392f1f241e5ad36316a8b79afef
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spelling	oai:doaj.org-article:5d710392f1f241e5ad36316a8b79afef2021-12-02T17:32:12Zd-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery10.1038/s41467-020-19709-62041-1723https://doaj.org/article/5d710392f1f241e5ad36316a8b79afef2020-11-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-19709-6https://doaj.org/toc/2041-1723Low intrinsic activity and accessibility of active sites limit the application of metal-organic framework as catalyst for Zn-air battery. Here, authors present a cation substitution strategy to regulate the electronic state of metal sites and modify its porosity, which enables battery operation.Yi JiangYa-Ping DengRuilin LiangJing FuRui GaoDan LuoZhengyu BaiYongfeng HuAiping YuZhongwei ChenNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-11 (2020)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Yi Jiang Ya-Ping Deng Ruilin Liang Jing Fu Rui Gao Dan Luo Zhengyu Bai Yongfeng Hu Aiping Yu Zhongwei Chen d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
description	Low intrinsic activity and accessibility of active sites limit the application of metal-organic framework as catalyst for Zn-air battery. Here, authors present a cation substitution strategy to regulate the electronic state of metal sites and modify its porosity, which enables battery operation.
format	article
author	Yi Jiang Ya-Ping Deng Ruilin Liang Jing Fu Rui Gao Dan Luo Zhengyu Bai Yongfeng Hu Aiping Yu Zhongwei Chen
author_facet	Yi Jiang Ya-Ping Deng Ruilin Liang Jing Fu Rui Gao Dan Luo Zhengyu Bai Yongfeng Hu Aiping Yu Zhongwei Chen
author_sort	Yi Jiang
title	d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
title_short	d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
title_full	d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
title_fullStr	d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
title_full_unstemmed	d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
title_sort	d-orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery
publisher	Nature Portfolio
publishDate	2020
url	https://doaj.org/article/5d710392f1f241e5ad36316a8b79afef
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d-Orbital steered active sites through ligand editing on heterometal imidazole frameworks for rechargeable zinc-air battery

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