Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation

Water oxidation to triplet oxygen requires a spin polarization process for faster kinetics. Here, the authors show an interface spin pinning effect between ferromagnetic oxides and reconstructed oxyhydroxide surface layer, where the spin ordering in paramagnetic oxyhydroxide catalyst layer can be tu...

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Autores principales: Tianze Wu, Xiao Ren, Yuanmiao Sun, Shengnan Sun, Guoyu Xian, Günther G. Scherer, Adrian C. Fisher, Daniel Mandler, Joel W. Ager, Alexis Grimaud, Junling Wang, Chengmin Shen, Haitao Yang, Jose Gracia, Hong-Jun Gao, Zhichuan J. Xu
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/5f1ab780d316472f8cbab4806ac313fa
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spelling oai:doaj.org-article:5f1ab780d316472f8cbab4806ac313fa2021-12-02T17:40:28ZSpin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation10.1038/s41467-021-23896-12041-1723https://doaj.org/article/5f1ab780d316472f8cbab4806ac313fa2021-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-23896-1https://doaj.org/toc/2041-1723Water oxidation to triplet oxygen requires a spin polarization process for faster kinetics. Here, the authors show an interface spin pinning effect between ferromagnetic oxides and reconstructed oxyhydroxide surface layer, where the spin ordering in paramagnetic oxyhydroxide catalyst layer can be tuned to improve the intrinsic activity.Tianze WuXiao RenYuanmiao SunShengnan SunGuoyu XianGünther G. SchererAdrian C. FisherDaniel MandlerJoel W. AgerAlexis GrimaudJunling WangChengmin ShenHaitao YangJose GraciaHong-Jun GaoZhichuan J. XuNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-11 (2021)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Tianze Wu
Xiao Ren
Yuanmiao Sun
Shengnan Sun
Guoyu Xian
Günther G. Scherer
Adrian C. Fisher
Daniel Mandler
Joel W. Ager
Alexis Grimaud
Junling Wang
Chengmin Shen
Haitao Yang
Jose Gracia
Hong-Jun Gao
Zhichuan J. Xu
Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
description Water oxidation to triplet oxygen requires a spin polarization process for faster kinetics. Here, the authors show an interface spin pinning effect between ferromagnetic oxides and reconstructed oxyhydroxide surface layer, where the spin ordering in paramagnetic oxyhydroxide catalyst layer can be tuned to improve the intrinsic activity.
format article
author Tianze Wu
Xiao Ren
Yuanmiao Sun
Shengnan Sun
Guoyu Xian
Günther G. Scherer
Adrian C. Fisher
Daniel Mandler
Joel W. Ager
Alexis Grimaud
Junling Wang
Chengmin Shen
Haitao Yang
Jose Gracia
Hong-Jun Gao
Zhichuan J. Xu
author_facet Tianze Wu
Xiao Ren
Yuanmiao Sun
Shengnan Sun
Guoyu Xian
Günther G. Scherer
Adrian C. Fisher
Daniel Mandler
Joel W. Ager
Alexis Grimaud
Junling Wang
Chengmin Shen
Haitao Yang
Jose Gracia
Hong-Jun Gao
Zhichuan J. Xu
author_sort Tianze Wu
title Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
title_short Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
title_full Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
title_fullStr Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
title_full_unstemmed Spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
title_sort spin pinning effect to reconstructed oxyhydroxide layer on ferromagnetic oxides for enhanced water oxidation
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/5f1ab780d316472f8cbab4806ac313fa
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