Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes

While cuprous oxide is a promising solar-to-fuel conversion material, photoelectrochemical devices substantially underperform. Here, the authors use femtosecond time-resolved two-photon photoemission spectroscopy to correlate photoexcited electron energetics and dynamics with performance losses.

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Autores principales: Mario Borgwardt, Stefan T. Omelchenko, Marco Favaro, Paul Plate, Christian Höhn, Daniel Abou-Ras, Klaus Schwarzburg, Roel van de Krol, Harry A. Atwater, Nathan S. Lewis, Rainer Eichberger, Dennis Friedrich
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Publicado: Nature Portfolio 2019
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Acceso en línea:https://doaj.org/article/63da452539ec41218ed9e6159992e34e
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spelling oai:doaj.org-article:63da452539ec41218ed9e6159992e34e2021-12-02T16:57:51ZFemtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes10.1038/s41467-019-10143-x2041-1723https://doaj.org/article/63da452539ec41218ed9e6159992e34e2019-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-10143-xhttps://doaj.org/toc/2041-1723While cuprous oxide is a promising solar-to-fuel conversion material, photoelectrochemical devices substantially underperform. Here, the authors use femtosecond time-resolved two-photon photoemission spectroscopy to correlate photoexcited electron energetics and dynamics with performance losses.Mario BorgwardtStefan T. OmelchenkoMarco FavaroPaul PlateChristian HöhnDaniel Abou-RasKlaus SchwarzburgRoel van de KrolHarry A. AtwaterNathan S. LewisRainer EichbergerDennis FriedrichNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-7 (2019)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Mario Borgwardt
Stefan T. Omelchenko
Marco Favaro
Paul Plate
Christian Höhn
Daniel Abou-Ras
Klaus Schwarzburg
Roel van de Krol
Harry A. Atwater
Nathan S. Lewis
Rainer Eichberger
Dennis Friedrich
Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
description While cuprous oxide is a promising solar-to-fuel conversion material, photoelectrochemical devices substantially underperform. Here, the authors use femtosecond time-resolved two-photon photoemission spectroscopy to correlate photoexcited electron energetics and dynamics with performance losses.
format article
author Mario Borgwardt
Stefan T. Omelchenko
Marco Favaro
Paul Plate
Christian Höhn
Daniel Abou-Ras
Klaus Schwarzburg
Roel van de Krol
Harry A. Atwater
Nathan S. Lewis
Rainer Eichberger
Dennis Friedrich
author_facet Mario Borgwardt
Stefan T. Omelchenko
Marco Favaro
Paul Plate
Christian Höhn
Daniel Abou-Ras
Klaus Schwarzburg
Roel van de Krol
Harry A. Atwater
Nathan S. Lewis
Rainer Eichberger
Dennis Friedrich
author_sort Mario Borgwardt
title Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
title_short Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
title_full Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
title_fullStr Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
title_full_unstemmed Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
title_sort femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in cu2o photoelectrodes
publisher Nature Portfolio
publishDate 2019
url https://doaj.org/article/63da452539ec41218ed9e6159992e34e
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AT rainereichberger femtosecondtimeresolvedtwophotonphotoemissionstudiesofultrafastcarrierrelaxationincu2ophotoelectrodes
AT dennisfriedrich femtosecondtimeresolvedtwophotonphotoemissionstudiesofultrafastcarrierrelaxationincu2ophotoelectrodes
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