Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes
While cuprous oxide is a promising solar-to-fuel conversion material, photoelectrochemical devices substantially underperform. Here, the authors use femtosecond time-resolved two-photon photoemission spectroscopy to correlate photoexcited electron energetics and dynamics with performance losses.
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Nature Portfolio
2019
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oai:doaj.org-article:63da452539ec41218ed9e6159992e34e2021-12-02T16:57:51ZFemtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes10.1038/s41467-019-10143-x2041-1723https://doaj.org/article/63da452539ec41218ed9e6159992e34e2019-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-10143-xhttps://doaj.org/toc/2041-1723While cuprous oxide is a promising solar-to-fuel conversion material, photoelectrochemical devices substantially underperform. Here, the authors use femtosecond time-resolved two-photon photoemission spectroscopy to correlate photoexcited electron energetics and dynamics with performance losses.Mario BorgwardtStefan T. OmelchenkoMarco FavaroPaul PlateChristian HöhnDaniel Abou-RasKlaus SchwarzburgRoel van de KrolHarry A. AtwaterNathan S. LewisRainer EichbergerDennis FriedrichNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-7 (2019) |
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Science Q Mario Borgwardt Stefan T. Omelchenko Marco Favaro Paul Plate Christian Höhn Daniel Abou-Ras Klaus Schwarzburg Roel van de Krol Harry A. Atwater Nathan S. Lewis Rainer Eichberger Dennis Friedrich Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes |
description |
While cuprous oxide is a promising solar-to-fuel conversion material, photoelectrochemical devices substantially underperform. Here, the authors use femtosecond time-resolved two-photon photoemission spectroscopy to correlate photoexcited electron energetics and dynamics with performance losses. |
format |
article |
author |
Mario Borgwardt Stefan T. Omelchenko Marco Favaro Paul Plate Christian Höhn Daniel Abou-Ras Klaus Schwarzburg Roel van de Krol Harry A. Atwater Nathan S. Lewis Rainer Eichberger Dennis Friedrich |
author_facet |
Mario Borgwardt Stefan T. Omelchenko Marco Favaro Paul Plate Christian Höhn Daniel Abou-Ras Klaus Schwarzburg Roel van de Krol Harry A. Atwater Nathan S. Lewis Rainer Eichberger Dennis Friedrich |
author_sort |
Mario Borgwardt |
title |
Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes |
title_short |
Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes |
title_full |
Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes |
title_fullStr |
Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes |
title_full_unstemmed |
Femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in Cu2O photoelectrodes |
title_sort |
femtosecond time-resolved two-photon photoemission studies of ultrafast carrier relaxation in cu2o photoelectrodes |
publisher |
Nature Portfolio |
publishDate |
2019 |
url |
https://doaj.org/article/63da452539ec41218ed9e6159992e34e |
work_keys_str_mv |
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_version_ |
1718382448709992448 |