All-XUV Pump-Probe Transient Absorption Spectroscopy of the Structural Molecular Dynamics of Di-iodomethane

All-XUV Pump-Probe Transient Absorption Spectroscopy of the Structural Molecular Dynamics of Di-iodomethane

In this work, we use an extreme-ultraviolet (XUV) free-electron laser (FEL) to resonantly excite the I: 4d_{5/2}–σ^{*} transition of a gas-phase di-iodomethane (CH_{2}I_{2}) target. This site-specific excitation generates a 4d core hole located at an iodine site, which leaves the molecule in a well-...

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Autores principales: Marc Rebholz, Thomas Ding, Victor Despré, Lennart Aufleger, Maximilian Hartmann, Kristina Meyer, Veit Stooß, Alexander Magunia, David Wachs, Paul Birk, Yonghao Mi, Gergana Dimitrova Borisova, Carina da Costa Castanheira, Patrick Rupprecht, Georg Schmid, Kirsten Schnorr, Claus Dieter Schröter, Robert Moshammer, Zhi-Heng Loh, Andrew R. Attar, Stephen R. Leone, Thomas Gaumnitz, Hans Jakob Wörner, Sebastian Roling, Marco Butz, Helmut Zacharias, Stefan Düsterer, Rolf Treusch, Günter Brenner, Jonas Vester, Alexander I. Kuleff, Christian Ott, Thomas Pfeifer
Formato: article
Lenguaje:EN
Publicado: American Physical Society 2021
Materias:
Physics
QC1-999
Acceso en línea:https://doaj.org/article/64b424a18119400eb2c7746afff63f50
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