Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}

The evolution between Fermi-liquid and non-Fermi-liquid states in correlated electron systems has been a central subject in condensed matter physics because of the coupled intriguing magnetic and electronic states. An effective pathway to explore the nature of non-Fermi-liquid behavior is to approac...

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Autores principales: Shengchun Shen, Zhuolu Li, Zijun Tian, Weidong Luo, Satoshi Okamoto, Pu Yu
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Lenguaje:EN
Publicado: American Physical Society 2021
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Acceso en línea:https://doaj.org/article/6511986db9444751bfcdffcb6c6b7af9
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spelling oai:doaj.org-article:6511986db9444751bfcdffcb6c6b7af92021-12-02T14:29:47ZEmergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}10.1103/PhysRevX.11.0210182160-3308https://doaj.org/article/6511986db9444751bfcdffcb6c6b7af92021-04-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.11.021018http://doi.org/10.1103/PhysRevX.11.021018https://doaj.org/toc/2160-3308The evolution between Fermi-liquid and non-Fermi-liquid states in correlated electron systems has been a central subject in condensed matter physics because of the coupled intriguing magnetic and electronic states. An effective pathway to explore the nature of non-Fermi-liquid behavior is to approach its phase boundary. Here we report a crossover from non-Fermi-liquid to Fermi-liquid state in metallic CaRuO_{3} through ionic liquid gating induced protonation with electric field. This electronic transition subsequently triggers a reversible magnetic transition with the emergence of an exotic ferromagnetic state from this paramagnetic compound. Our theoretical analysis reveals that hydrogen incorporation plays a critical role in both the electronic and magnetic phase transitions via structural distortion and electron doping. These observations not only help understand the correlated magnetic and electronic transitions in perovskite ruthenate systems, but also provide novel pathways to design electronic phases in correlated materials.Shengchun ShenZhuolu LiZijun TianWeidong LuoSatoshi OkamotoPu YuAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 11, Iss 2, p 021018 (2021)
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
spellingShingle Physics
QC1-999
Shengchun Shen
Zhuolu Li
Zijun Tian
Weidong Luo
Satoshi Okamoto
Pu Yu
Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}
description The evolution between Fermi-liquid and non-Fermi-liquid states in correlated electron systems has been a central subject in condensed matter physics because of the coupled intriguing magnetic and electronic states. An effective pathway to explore the nature of non-Fermi-liquid behavior is to approach its phase boundary. Here we report a crossover from non-Fermi-liquid to Fermi-liquid state in metallic CaRuO_{3} through ionic liquid gating induced protonation with electric field. This electronic transition subsequently triggers a reversible magnetic transition with the emergence of an exotic ferromagnetic state from this paramagnetic compound. Our theoretical analysis reveals that hydrogen incorporation plays a critical role in both the electronic and magnetic phase transitions via structural distortion and electron doping. These observations not only help understand the correlated magnetic and electronic transitions in perovskite ruthenate systems, but also provide novel pathways to design electronic phases in correlated materials.
format article
author Shengchun Shen
Zhuolu Li
Zijun Tian
Weidong Luo
Satoshi Okamoto
Pu Yu
author_facet Shengchun Shen
Zhuolu Li
Zijun Tian
Weidong Luo
Satoshi Okamoto
Pu Yu
author_sort Shengchun Shen
title Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}
title_short Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}
title_full Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}
title_fullStr Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}
title_full_unstemmed Emergent Ferromagnetism with Fermi-Liquid Behavior in Proton Intercalated CaRuO_{3}
title_sort emergent ferromagnetism with fermi-liquid behavior in proton intercalated caruo_{3}
publisher American Physical Society
publishDate 2021
url https://doaj.org/article/6511986db9444751bfcdffcb6c6b7af9
work_keys_str_mv AT shengchunshen emergentferromagnetismwithfermiliquidbehaviorinprotonintercalatedcaruo3
AT zhuoluli emergentferromagnetismwithfermiliquidbehaviorinprotonintercalatedcaruo3
AT zijuntian emergentferromagnetismwithfermiliquidbehaviorinprotonintercalatedcaruo3
AT weidongluo emergentferromagnetismwithfermiliquidbehaviorinprotonintercalatedcaruo3
AT satoshiokamoto emergentferromagnetismwithfermiliquidbehaviorinprotonintercalatedcaruo3
AT puyu emergentferromagnetismwithfermiliquidbehaviorinprotonintercalatedcaruo3
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