Multiple quantum phase transitions of different nature in the topological kagome magnet Co3Sn2−x In x S2

Abstract The exploration of topological electronic phases that result from strong electronic correlations is a frontier in condensed matter physics. One class of systems that is currently emerging as a platform for such studies are so-called kagome magnets based on transition metals. Using muon spin...

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Autores principales: Z. Guguchia, H. Zhou, C. N. Wang, J.-X. Yin, C. Mielke, S. S. Tsirkin, I. Belopolski, S.-S. Zhang, T. A. Cochran, T. Neupert, R. Khasanov, A. Amato, S. Jia, M. Z. Hasan, H. Luetkens
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/66c114d864b2491ea5adb4b7cf2b2345
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Sumario:Abstract The exploration of topological electronic phases that result from strong electronic correlations is a frontier in condensed matter physics. One class of systems that is currently emerging as a platform for such studies are so-called kagome magnets based on transition metals. Using muon spin-rotation, we explore magnetic correlations in the kagome magnet Co3Sn2−xInxS2 as a function of In-doping, providing putative evidence for an intriguing incommensurate helimagnetic (HM) state. Our results show that, while the undoped sample exhibits an out-of-plane ferromagnetic (FM) ground state, at 5% of In-doping the system enters a state in which FM and in-plane antiferromagnetic (AFM) phases coexist. At higher doping, a HM state emerges and becomes dominant at the critical doping level of only x cr,1 ≃ 0.3. This indicates a zero temperature first order quantum phase transition from the FM, through a mixed state, to a helical phase at x cr,1. In addition, at x cr,2 ≃ 1, a zero temperature second order phase transition from helical to paramagnetic phase is observed, evidencing a HM quantum critical point (QCP) in the phase diagram of the topological magnet Co3Sn2−xInxS2. The observed diversity of interactions in the magnetic kagome lattice drives non-monotonous variations of the topological Hall response of this system.