Atomic layer confined vacancies for atomic-level insights into carbon dioxide electroreduction

The role of oxygen vacancies in carbon dioxide reduction remains somewhat unclear. Here, the authors fabricate vacancy-rich and vacancy-poor Co3O4single-unit-cell layers, and demonstrate by X-ray absorption and DFT that the material is a promising platform for mechanistic studies of carbon dioxide r...

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Auteurs principaux: Shan Gao, Zhongti Sun, Wei Liu, Xingchen Jiao, Xiaolong Zu, Qitao Hu, Yongfu Sun, Tao Yao, Wenhua Zhang, Shiqiang Wei, Yi Xie
Format: article
Langue:EN
Publié: Nature Portfolio 2017
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Accès en ligne:https://doaj.org/article/6723845d98d0453a99371d85cc9b4da0
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Résumé:The role of oxygen vacancies in carbon dioxide reduction remains somewhat unclear. Here, the authors fabricate vacancy-rich and vacancy-poor Co3O4single-unit-cell layers, and demonstrate by X-ray absorption and DFT that the material is a promising platform for mechanistic studies of carbon dioxide reduction.