Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase

Abstract Nanoparticles composed of multiple silver cores and a plasma polymer shell (multicore@shell) were prepared in a single step with a gas aggregation cluster source operating with Ar/hexamethyldisiloxane mixtures and optionally oxygen. The size distribution of the metal inclusions as well as t...

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Autores principales: Pavel Solař, Oleksandr Polonskyi, Ansgar Olbricht, Alexander Hinz, Artem Shelemin, Ondřej Kylián, Andrei Choukourov, Franz Faupel, Hynek Biederman
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/6a1350deb9054681bf08cc4343681895
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spelling oai:doaj.org-article:6a1350deb9054681bf08cc43436818952021-12-02T11:52:56ZSingle-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase10.1038/s41598-017-08274-62045-2322https://doaj.org/article/6a1350deb9054681bf08cc43436818952017-08-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-08274-6https://doaj.org/toc/2045-2322Abstract Nanoparticles composed of multiple silver cores and a plasma polymer shell (multicore@shell) were prepared in a single step with a gas aggregation cluster source operating with Ar/hexamethyldisiloxane mixtures and optionally oxygen. The size distribution of the metal inclusions as well as the chemical composition and the thickness of the shells were found to be controlled by the composition of the working gas mixture. Shell matrices ranging from organosilicon plasma polymer to nearly stoichiometric SiO2 were obtained. The method allows facile fabrication of multicore@shell nanoparticles with tailored functional properties, as demonstrated here with the optical response.Pavel SolařOleksandr PolonskyiAnsgar OlbrichtAlexander HinzArtem SheleminOndřej KyliánAndrei ChoukourovFranz FaupelHynek BiedermanNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-6 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Pavel Solař
Oleksandr Polonskyi
Ansgar Olbricht
Alexander Hinz
Artem Shelemin
Ondřej Kylián
Andrei Choukourov
Franz Faupel
Hynek Biederman
Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
description Abstract Nanoparticles composed of multiple silver cores and a plasma polymer shell (multicore@shell) were prepared in a single step with a gas aggregation cluster source operating with Ar/hexamethyldisiloxane mixtures and optionally oxygen. The size distribution of the metal inclusions as well as the chemical composition and the thickness of the shells were found to be controlled by the composition of the working gas mixture. Shell matrices ranging from organosilicon plasma polymer to nearly stoichiometric SiO2 were obtained. The method allows facile fabrication of multicore@shell nanoparticles with tailored functional properties, as demonstrated here with the optical response.
format article
author Pavel Solař
Oleksandr Polonskyi
Ansgar Olbricht
Alexander Hinz
Artem Shelemin
Ondřej Kylián
Andrei Choukourov
Franz Faupel
Hynek Biederman
author_facet Pavel Solař
Oleksandr Polonskyi
Ansgar Olbricht
Alexander Hinz
Artem Shelemin
Ondřej Kylián
Andrei Choukourov
Franz Faupel
Hynek Biederman
author_sort Pavel Solař
title Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
title_short Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
title_full Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
title_fullStr Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
title_full_unstemmed Single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
title_sort single-step generation of metal-plasma polymer multicore@shell nanoparticles from the gas phase
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/6a1350deb9054681bf08cc4343681895
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