Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy

Photo-excited charge carrier dynamics in photocatalytic materials with rough surfaces have been studied via measurements using pattern-illumination time-resolved phase microscopy. Optimal defocusing is necessary for the phase-contrast detection of the refractive index change due to the photo-excited...

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Autores principales: Kenji Katayama, Tatsuya Chugenji, Kei Kawaguchi
Formato: article
Lenguaje:EN
Publicado: AIP Publishing LLC 2021
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Acceso en línea:https://doaj.org/article/6ab73b2e172243cbb73ea4a5504baf31
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spelling oai:doaj.org-article:6ab73b2e172243cbb73ea4a5504baf312021-12-01T18:52:06ZDefocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy2158-322610.1063/5.0072245https://doaj.org/article/6ab73b2e172243cbb73ea4a5504baf312021-11-01T00:00:00Zhttp://dx.doi.org/10.1063/5.0072245https://doaj.org/toc/2158-3226Photo-excited charge carrier dynamics in photocatalytic materials with rough surfaces have been studied via measurements using pattern-illumination time-resolved phase microscopy. Optimal defocusing is necessary for the phase-contrast detection of the refractive index change due to the photo-excited charge carriers. The signal enhancement of the phase-change was explained theoretically and experimentally. The optical phase variation due to the transmission of a rough surface is coupled with the quadratic phase term in Fresnel diffraction, and a slight defocusing can convert the phase image to the corresponding amplitude image. The phase-contrast image due to the photo-excited charge carriers is also enhanced by the defocusing. The explanation was supported by wave optics calculation, and the enhancement was demonstrated for two types of TiO2 substrates with different roughnesses.Kenji KatayamaTatsuya ChugenjiKei KawaguchiAIP Publishing LLCarticlePhysicsQC1-999ENAIP Advances, Vol 11, Iss 11, Pp 115215-115215-7 (2021)
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
spellingShingle Physics
QC1-999
Kenji Katayama
Tatsuya Chugenji
Kei Kawaguchi
Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
description Photo-excited charge carrier dynamics in photocatalytic materials with rough surfaces have been studied via measurements using pattern-illumination time-resolved phase microscopy. Optimal defocusing is necessary for the phase-contrast detection of the refractive index change due to the photo-excited charge carriers. The signal enhancement of the phase-change was explained theoretically and experimentally. The optical phase variation due to the transmission of a rough surface is coupled with the quadratic phase term in Fresnel diffraction, and a slight defocusing can convert the phase image to the corresponding amplitude image. The phase-contrast image due to the photo-excited charge carriers is also enhanced by the defocusing. The explanation was supported by wave optics calculation, and the enhancement was demonstrated for two types of TiO2 substrates with different roughnesses.
format article
author Kenji Katayama
Tatsuya Chugenji
Kei Kawaguchi
author_facet Kenji Katayama
Tatsuya Chugenji
Kei Kawaguchi
author_sort Kenji Katayama
title Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
title_short Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
title_full Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
title_fullStr Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
title_full_unstemmed Defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
title_sort defocus-induced phase contrast enhancement in pattern illumination time-resolved phase microscopy
publisher AIP Publishing LLC
publishDate 2021
url https://doaj.org/article/6ab73b2e172243cbb73ea4a5504baf31
work_keys_str_mv AT kenjikatayama defocusinducedphasecontrastenhancementinpatternilluminationtimeresolvedphasemicroscopy
AT tatsuyachugenji defocusinducedphasecontrastenhancementinpatternilluminationtimeresolvedphasemicroscopy
AT keikawaguchi defocusinducedphasecontrastenhancementinpatternilluminationtimeresolvedphasemicroscopy
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