17O-EPR determination of the structure and dynamics of copper single-metal sites in zeolites

The identification of catalytically active sites with atomic-scale precision occupies a central place in the theory and practice of heterogeneous catalysis. Here the authors assess the nature of the copper-oxygen bond in a Cu-CHA zeolite and recover the microscopic structure of single-metal sites.

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Bibliographic Details
Main Authors: Paolo Cleto Bruzzese, Enrico Salvadori, Stefan Jäger, Martin Hartmann, Bartolomeo Civalleri, Andreas Pöppl, Mario Chiesa
Format: article
Language:EN
Published: Nature Portfolio 2021
Subjects:
Q
Online Access:https://doaj.org/article/6b5ffe4dd8ae4edab23d5e85b1577912
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Summary:The identification of catalytically active sites with atomic-scale precision occupies a central place in the theory and practice of heterogeneous catalysis. Here the authors assess the nature of the copper-oxygen bond in a Cu-CHA zeolite and recover the microscopic structure of single-metal sites.