Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%

Abstract Poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) mixed with single-wall nanotubes (SWNTs) (10:1) and doped with (0.1 M) perchloric acid (HClO4) in a solution-processed film, working as an excellent thin transparent conducting film (TCF) in organic solar cells, was investig...

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Autores principales: S. Wageh, Mahfoudh Raïssi, Thomas Berthelot, Matthieu Laurent, Didier Rousseau, Abdullah M. Abusorrah, Omar A. Al-Hartomy, Ahmed A. Al-Ghamdi
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Publicado: Nature Portfolio 2021
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spelling oai:doaj.org-article:6ffeb6377e0e4cd8bd988179402f5a532021-12-02T15:39:41ZDigital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%10.1038/s41598-021-93365-82045-2322https://doaj.org/article/6ffeb6377e0e4cd8bd988179402f5a532021-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-93365-8https://doaj.org/toc/2045-2322Abstract Poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) mixed with single-wall nanotubes (SWNTs) (10:1) and doped with (0.1 M) perchloric acid (HClO4) in a solution-processed film, working as an excellent thin transparent conducting film (TCF) in organic solar cells, was investigated. This new electrode structure can be an outstanding substitute for conventional indium tin oxide (ITO) for applications in flexible solar cells due to the potential of attaining high transparency with enhanced conductivity, good flexibility, and good durability via a low-cost process over a large area. In addition, solution-processed vanadium oxide (VOx) doped with a small amount of PEDOT-PSS(PH1000) can be applied as a hole transport layer (HTL) for achieving high efficiency and stability. From these viewpoints, we investigate the benefit of using printed SWNTs-PEDOT-PSS doped with HClO4 as a transparent conducting electrode in a flexible organic solar cell. Additionally, we applied a VOx-PEDOT-PSS thin film as a hole transporting layer and a blend of PTB7 (polythieno[3,4-b] thiophene/benzodithiophene): PC71BM (phenyl-C71-butyric acid methyl ester) as an active layer in devices. Zinc oxide (ZnO) nanoparticles were applied as an electron transport layer and Ag was used as the top electrode. The proposed solar cell structure showed an enhancement in short-circuit current, power conversion efficiency, and stability relative to a conventional cell based on ITO. This result suggests a great carrier injection throughout the interfacial layer, high conductivity and transparency, as well as firm adherence for the new electrode.S. WagehMahfoudh RaïssiThomas BerthelotMatthieu LaurentDidier RousseauAbdullah M. AbusorrahOmar A. Al-HartomyAhmed A. Al-GhamdiNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-16 (2021)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
S. Wageh
Mahfoudh Raïssi
Thomas Berthelot
Matthieu Laurent
Didier Rousseau
Abdullah M. Abusorrah
Omar A. Al-Hartomy
Ahmed A. Al-Ghamdi
Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
description Abstract Poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) mixed with single-wall nanotubes (SWNTs) (10:1) and doped with (0.1 M) perchloric acid (HClO4) in a solution-processed film, working as an excellent thin transparent conducting film (TCF) in organic solar cells, was investigated. This new electrode structure can be an outstanding substitute for conventional indium tin oxide (ITO) for applications in flexible solar cells due to the potential of attaining high transparency with enhanced conductivity, good flexibility, and good durability via a low-cost process over a large area. In addition, solution-processed vanadium oxide (VOx) doped with a small amount of PEDOT-PSS(PH1000) can be applied as a hole transport layer (HTL) for achieving high efficiency and stability. From these viewpoints, we investigate the benefit of using printed SWNTs-PEDOT-PSS doped with HClO4 as a transparent conducting electrode in a flexible organic solar cell. Additionally, we applied a VOx-PEDOT-PSS thin film as a hole transporting layer and a blend of PTB7 (polythieno[3,4-b] thiophene/benzodithiophene): PC71BM (phenyl-C71-butyric acid methyl ester) as an active layer in devices. Zinc oxide (ZnO) nanoparticles were applied as an electron transport layer and Ag was used as the top electrode. The proposed solar cell structure showed an enhancement in short-circuit current, power conversion efficiency, and stability relative to a conventional cell based on ITO. This result suggests a great carrier injection throughout the interfacial layer, high conductivity and transparency, as well as firm adherence for the new electrode.
format article
author S. Wageh
Mahfoudh Raïssi
Thomas Berthelot
Matthieu Laurent
Didier Rousseau
Abdullah M. Abusorrah
Omar A. Al-Hartomy
Ahmed A. Al-Ghamdi
author_facet S. Wageh
Mahfoudh Raïssi
Thomas Berthelot
Matthieu Laurent
Didier Rousseau
Abdullah M. Abusorrah
Omar A. Al-Hartomy
Ahmed A. Al-Ghamdi
author_sort S. Wageh
title Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
title_short Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
title_full Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
title_fullStr Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
title_full_unstemmed Digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
title_sort digital printing of a novel electrode for stable flexible organic solar cells with a power conversion efficiency of 8.5%
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/6ffeb6377e0e4cd8bd988179402f5a53
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