CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters

Platinum nanocatalysts play critical roles in CO oxidation. Herein, the authors discover that under-coordinated Pt atoms at the edges of the first cluster layer are rendered cationic by direct contact with the Al2O3 support, which affects the overall CO oxidation activity.

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Autores principales:	Atsushi Beniya, Shougo Higashi, Nobuko Ohba, Ryosuke Jinnouchi, Hirohito Hirata, Yoshihide Watanabe
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2020
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/702dbe45edea45f18d67cc64163417fc
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spelling	oai:doaj.org-article:702dbe45edea45f18d67cc64163417fc2021-12-02T15:39:17ZCO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters10.1038/s41467-020-15850-42041-1723https://doaj.org/article/702dbe45edea45f18d67cc64163417fc2020-04-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-15850-4https://doaj.org/toc/2041-1723Platinum nanocatalysts play critical roles in CO oxidation. Herein, the authors discover that under-coordinated Pt atoms at the edges of the first cluster layer are rendered cationic by direct contact with the Al2O3 support, which affects the overall CO oxidation activity.Atsushi BeniyaShougo HigashiNobuko OhbaRyosuke JinnouchiHirohito HirataYoshihide WatanabeNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-10 (2020)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Atsushi Beniya Shougo Higashi Nobuko Ohba Ryosuke Jinnouchi Hirohito Hirata Yoshihide Watanabe CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters
description	Platinum nanocatalysts play critical roles in CO oxidation. Herein, the authors discover that under-coordinated Pt atoms at the edges of the first cluster layer are rendered cationic by direct contact with the Al2O3 support, which affects the overall CO oxidation activity.
format	article
author	Atsushi Beniya Shougo Higashi Nobuko Ohba Ryosuke Jinnouchi Hirohito Hirata Yoshihide Watanabe
author_facet	Atsushi Beniya Shougo Higashi Nobuko Ohba Ryosuke Jinnouchi Hirohito Hirata Yoshihide Watanabe
author_sort	Atsushi Beniya
title	CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters
title_short	CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters
title_full	CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters
title_fullStr	CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters
title_full_unstemmed	CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters
title_sort	co oxidation activity of non-reducible oxide-supported mass-selected few-atom pt single-clusters
publisher	Nature Portfolio
publishDate	2020
url	https://doaj.org/article/702dbe45edea45f18d67cc64163417fc
work_keys_str_mv	AT atsushibeniya cooxidationactivityofnonreducibleoxidesupportedmassselectedfewatomptsingleclusters AT shougohigashi cooxidationactivityofnonreducibleoxidesupportedmassselectedfewatomptsingleclusters AT nobukoohba cooxidationactivityofnonreducibleoxidesupportedmassselectedfewatomptsingleclusters AT ryosukejinnouchi cooxidationactivityofnonreducibleoxidesupportedmassselectedfewatomptsingleclusters AT hirohitohirata cooxidationactivityofnonreducibleoxidesupportedmassselectedfewatomptsingleclusters AT yoshihidewatanabe cooxidationactivityofnonreducibleoxidesupportedmassselectedfewatomptsingleclusters
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CO oxidation activity of non-reducible oxide-supported mass-selected few-atom Pt single-clusters

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