Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction
Abstract MXenes, an emerging two-dimensional (2D) transition metal carbides, nitrides and carbonitrides, have exhibited great potential as electrocatalysts for hydrogen evolution reaction (HER) due to the excellent characters, including excellent structural and chemical stability, superior electrica...
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2021
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oai:doaj.org-article:74eec4bbc26a4c629eb5a88b923602d22021-12-02T19:12:34ZRecent advances of MXenes as electrocatalysts for hydrogen evolution reaction10.1038/s41699-021-00259-42397-7132https://doaj.org/article/74eec4bbc26a4c629eb5a88b923602d22021-09-01T00:00:00Zhttps://doi.org/10.1038/s41699-021-00259-4https://doaj.org/toc/2397-7132Abstract MXenes, an emerging two-dimensional (2D) transition metal carbides, nitrides and carbonitrides, have exhibited great potential as electrocatalysts for hydrogen evolution reaction (HER) due to the excellent characters, including excellent structural and chemical stability, superior electrical conductivity, and large active surface area. In this comprehensive study, firstly, the preparation advances of MXenes are systematically summarized. Then, the representative applications of MXenes-based HER electrocatalysts are introduced, from experimental and theoretical aspects. Thirdly, the strategies for improving HER catalytic activity of MXenes are demonstrated, such as optimizing active sites by termination modification and metal-atom doping, increasing active sites by fabricating various nanostructures. Finally, the existing challenges and new opportunities for MXenes-based electrocatalysts are also elucidated. This paper provides reference for the future development of new and efficient MXenes-based electrocatalysts for hydrogen production through water-splitting technology.Saishuai BaiMeiqing YangJizhou JiangXiaomiao HeJing ZouZhiguo XiongGuodong LiaoSong LiuNature PortfolioarticleMaterials of engineering and construction. Mechanics of materialsTA401-492ChemistryQD1-999ENnpj 2D Materials and Applications, Vol 5, Iss 1, Pp 1-15 (2021) |
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Materials of engineering and construction. Mechanics of materials TA401-492 Chemistry QD1-999 |
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Materials of engineering and construction. Mechanics of materials TA401-492 Chemistry QD1-999 Saishuai Bai Meiqing Yang Jizhou Jiang Xiaomiao He Jing Zou Zhiguo Xiong Guodong Liao Song Liu Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction |
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Abstract MXenes, an emerging two-dimensional (2D) transition metal carbides, nitrides and carbonitrides, have exhibited great potential as electrocatalysts for hydrogen evolution reaction (HER) due to the excellent characters, including excellent structural and chemical stability, superior electrical conductivity, and large active surface area. In this comprehensive study, firstly, the preparation advances of MXenes are systematically summarized. Then, the representative applications of MXenes-based HER electrocatalysts are introduced, from experimental and theoretical aspects. Thirdly, the strategies for improving HER catalytic activity of MXenes are demonstrated, such as optimizing active sites by termination modification and metal-atom doping, increasing active sites by fabricating various nanostructures. Finally, the existing challenges and new opportunities for MXenes-based electrocatalysts are also elucidated. This paper provides reference for the future development of new and efficient MXenes-based electrocatalysts for hydrogen production through water-splitting technology. |
format |
article |
author |
Saishuai Bai Meiqing Yang Jizhou Jiang Xiaomiao He Jing Zou Zhiguo Xiong Guodong Liao Song Liu |
author_facet |
Saishuai Bai Meiqing Yang Jizhou Jiang Xiaomiao He Jing Zou Zhiguo Xiong Guodong Liao Song Liu |
author_sort |
Saishuai Bai |
title |
Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction |
title_short |
Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction |
title_full |
Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction |
title_fullStr |
Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction |
title_full_unstemmed |
Recent advances of MXenes as electrocatalysts for hydrogen evolution reaction |
title_sort |
recent advances of mxenes as electrocatalysts for hydrogen evolution reaction |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/74eec4bbc26a4c629eb5a88b923602d2 |
work_keys_str_mv |
AT saishuaibai recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT meiqingyang recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT jizhoujiang recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT xiaomiaohe recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT jingzou recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT zhiguoxiong recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT guodongliao recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction AT songliu recentadvancesofmxenesaselectrocatalystsforhydrogenevolutionreaction |
_version_ |
1718377021620355072 |