Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices

Abstract Artificial superlattices constructed with ferromagnetic La0.7Sr0.3MnO3 layer and ferroelectric Ba0.7Sr0.3TiO3 layer were designed and fabricated on SrTiO3 substrates. An epitaxial growth with sharp interfaces between La0.7Sr0.3MnO3 and Ba0.7Sr0.3TiO3 layers was confirmed by scanning transmi...

Descripción completa

Guardado en:

Detalles Bibliográficos
Autores principales:	Haizhong Guo, Qingqing Li, Zhengzhong Yang, Kui-juan Jin, Chen Ge, Lin Gu, Xu He, Xiaolong Li, Ruiqiang Zhao, Qian Wan, Jiesu Wang, Meng He, Can Wang, Huibin Lu, Yuping Yang, Guozhen Yang
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2017
Materias:	Medicine R Science Q
Acceso en línea:	https://doaj.org/article/74f00d64a80c404ead77be23dd71e721
Etiquetas:	Agregar Etiqueta Sin Etiquetas, Sea el primero en etiquetar este registro!

id	oai:doaj.org-article:74f00d64a80c404ead77be23dd71e721
record_format	dspace
spelling	oai:doaj.org-article:74f00d64a80c404ead77be23dd71e7212021-12-02T16:06:57ZManipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices10.1038/s41598-017-08260-y2045-2322https://doaj.org/article/74f00d64a80c404ead77be23dd71e7212017-08-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-08260-yhttps://doaj.org/toc/2045-2322Abstract Artificial superlattices constructed with ferromagnetic La0.7Sr0.3MnO3 layer and ferroelectric Ba0.7Sr0.3TiO3 layer were designed and fabricated on SrTiO3 substrates. An epitaxial growth with sharp interfaces between La0.7Sr0.3MnO3 and Ba0.7Sr0.3TiO3 layers was confirmed by scanning transmission electron microscopy and x-ray diffraction. An unambiguous charge transfer involving an electron transferring from the La0.7Sr0.3MnO3 layers to Ba0.7Sr0.3TiO3 layers (Mn3+→Mn4+; Ti4+→Ti3+) across the interface were resolved by electron energy loss spectra analysis. These observations are attributed to the possible modification in the stereochemistry of the Ti and Mn ions in the interfacial region. The out-of-plane lattice parameter, Curie temperature, and magnetoresistance are strongly affected by the thicknesses of the La0.7Sr0.3MnO3 and Ba0.7Sr0.3TiO3 layers. Huge magnetoresistance subsisting to low temperature was also observed in the La0.7Sr0.3MnO3/Ba0.7Sr0.3TiO3 superlattices. All spectral changes identified at a nanometer scale and their potential effect on the degradation of magnetic and transport properties at a macroscopic level. These findings highlight the importance of dependence on sublayer thickness, illustrating the high degree of tenability in these artificially low-dimensional oxide materials.Haizhong GuoQingqing LiZhengzhong YangKui-juan JinChen GeLin GuXu HeXiaolong LiRuiqiang ZhaoQian WanJiesu WangMeng HeCan WangHuibin LuYuping YangGuozhen YangNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-11 (2017)
institution	DOAJ
collection	DOAJ
language	EN
topic	Medicine R Science Q
spellingShingle	Medicine R Science Q Haizhong Guo Qingqing Li Zhengzhong Yang Kui-juan Jin Chen Ge Lin Gu Xu He Xiaolong Li Ruiqiang Zhao Qian Wan Jiesu Wang Meng He Can Wang Huibin Lu Yuping Yang Guozhen Yang Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices
description	Abstract Artificial superlattices constructed with ferromagnetic La0.7Sr0.3MnO3 layer and ferroelectric Ba0.7Sr0.3TiO3 layer were designed and fabricated on SrTiO3 substrates. An epitaxial growth with sharp interfaces between La0.7Sr0.3MnO3 and Ba0.7Sr0.3TiO3 layers was confirmed by scanning transmission electron microscopy and x-ray diffraction. An unambiguous charge transfer involving an electron transferring from the La0.7Sr0.3MnO3 layers to Ba0.7Sr0.3TiO3 layers (Mn3+→Mn4+; Ti4+→Ti3+) across the interface were resolved by electron energy loss spectra analysis. These observations are attributed to the possible modification in the stereochemistry of the Ti and Mn ions in the interfacial region. The out-of-plane lattice parameter, Curie temperature, and magnetoresistance are strongly affected by the thicknesses of the La0.7Sr0.3MnO3 and Ba0.7Sr0.3TiO3 layers. Huge magnetoresistance subsisting to low temperature was also observed in the La0.7Sr0.3MnO3/Ba0.7Sr0.3TiO3 superlattices. All spectral changes identified at a nanometer scale and their potential effect on the degradation of magnetic and transport properties at a macroscopic level. These findings highlight the importance of dependence on sublayer thickness, illustrating the high degree of tenability in these artificially low-dimensional oxide materials.
format	article
author	Haizhong Guo Qingqing Li Zhengzhong Yang Kui-juan Jin Chen Ge Lin Gu Xu He Xiaolong Li Ruiqiang Zhao Qian Wan Jiesu Wang Meng He Can Wang Huibin Lu Yuping Yang Guozhen Yang
author_facet	Haizhong Guo Qingqing Li Zhengzhong Yang Kui-juan Jin Chen Ge Lin Gu Xu He Xiaolong Li Ruiqiang Zhao Qian Wan Jiesu Wang Meng He Can Wang Huibin Lu Yuping Yang Guozhen Yang
author_sort	Haizhong Guo
title	Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices
title_short	Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices
title_full	Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices
title_fullStr	Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices
title_full_unstemmed	Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices
title_sort	manipulating magnetoelectric properties by interfacial coupling in la0.3sr0.7mno3/ba0.7sr0.3tio3 superlattices
publisher	Nature Portfolio
publishDate	2017
url	https://doaj.org/article/74f00d64a80c404ead77be23dd71e721
work_keys_str_mv	AT haizhongguo manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT qingqingli manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT zhengzhongyang manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT kuijuanjin manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT chenge manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT lingu manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT xuhe manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT xiaolongli manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT ruiqiangzhao manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT qianwan manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT jiesuwang manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT menghe manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT canwang manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT huibinlu manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT yupingyang manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices AT guozhenyang manipulatingmagnetoelectricpropertiesbyinterfacialcouplinginla03sr07mno3ba07sr03tio3superlattices
_version_	1718384783124332544

Manipulating magnetoelectric properties by interfacial coupling in La0.3Sr0.7MnO3/Ba0.7Sr0.3TiO3 superlattices

Ejemplares similares