Adjacent single-atom irons boosting molecular oxygen activation on MnO2

Efficient oxygen activation is crucial for catalytic oxidation reaction, but highly depends on the construction of active sites. Here, dual adjacent Fe atoms anchored on MnO2 can assemble into a diatomic site, which activates molecular oxygen to form an active intermediate species Fe(O = O)Fe for CO...

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Autores principales:	Huayu Gu, Xiao Liu, Xiufan Liu, Cancan Ling, Kai Wei, Guangming Zhan, Yanbing Guo, Lizhi Zhang
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2021
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/7ab6b1fd8966410aa5c0660ae7b52abb
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spelling	oai:doaj.org-article:7ab6b1fd8966410aa5c0660ae7b52abb2021-12-02T18:02:16ZAdjacent single-atom irons boosting molecular oxygen activation on MnO210.1038/s41467-021-25726-w2041-1723https://doaj.org/article/7ab6b1fd8966410aa5c0660ae7b52abb2021-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-25726-whttps://doaj.org/toc/2041-1723Efficient oxygen activation is crucial for catalytic oxidation reaction, but highly depends on the construction of active sites. Here, dual adjacent Fe atoms anchored on MnO2 can assemble into a diatomic site, which activates molecular oxygen to form an active intermediate species Fe(O = O)Fe for CO oxidation.Huayu GuXiao LiuXiufan LiuCancan LingKai WeiGuangming ZhanYanbing GuoLizhi ZhangNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Huayu Gu Xiao Liu Xiufan Liu Cancan Ling Kai Wei Guangming Zhan Yanbing Guo Lizhi Zhang Adjacent single-atom irons boosting molecular oxygen activation on MnO2
description	Efficient oxygen activation is crucial for catalytic oxidation reaction, but highly depends on the construction of active sites. Here, dual adjacent Fe atoms anchored on MnO2 can assemble into a diatomic site, which activates molecular oxygen to form an active intermediate species Fe(O = O)Fe for CO oxidation.
format	article
author	Huayu Gu Xiao Liu Xiufan Liu Cancan Ling Kai Wei Guangming Zhan Yanbing Guo Lizhi Zhang
author_facet	Huayu Gu Xiao Liu Xiufan Liu Cancan Ling Kai Wei Guangming Zhan Yanbing Guo Lizhi Zhang
author_sort	Huayu Gu
title	Adjacent single-atom irons boosting molecular oxygen activation on MnO2
title_short	Adjacent single-atom irons boosting molecular oxygen activation on MnO2
title_full	Adjacent single-atom irons boosting molecular oxygen activation on MnO2
title_fullStr	Adjacent single-atom irons boosting molecular oxygen activation on MnO2
title_full_unstemmed	Adjacent single-atom irons boosting molecular oxygen activation on MnO2
title_sort	adjacent single-atom irons boosting molecular oxygen activation on mno2
publisher	Nature Portfolio
publishDate	2021
url	https://doaj.org/article/7ab6b1fd8966410aa5c0660ae7b52abb
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Adjacent single-atom irons boosting molecular oxygen activation on MnO2

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