A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles

This work investigates the mechanical properties, microstructures, and water-swelling behavior of a novel hydrogel filled with magnetic particles. The nanoparticles of magnetite (Fe<sub>3</sub>O<sub>4</sub>) and the micro-particles of carbonyl iron (CI) were selected and fill...

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Autores principales: Chanchan Xu, Bin Li, Xiaojie Wang
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Lenguaje:EN
Publicado: MDPI AG 2021
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Acceso en línea:https://doaj.org/article/7cb01f2fad3b45b0935c8447bfd9c732
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spelling oai:doaj.org-article:7cb01f2fad3b45b0935c8447bfd9c7322021-11-25T17:55:34ZA Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles10.3390/ijms2222123421422-00671661-6596https://doaj.org/article/7cb01f2fad3b45b0935c8447bfd9c7322021-11-01T00:00:00Zhttps://www.mdpi.com/1422-0067/22/22/12342https://doaj.org/toc/1661-6596https://doaj.org/toc/1422-0067This work investigates the mechanical properties, microstructures, and water-swelling behavior of a novel hydrogel filled with magnetic particles. The nanoparticles of magnetite (Fe<sub>3</sub>O<sub>4</sub>) and the micro-particles of carbonyl iron (CI) were selected and filled into a polyacrylamide (PAAM) hydrogel matrix to create two types of magnetic hydrogels. The isotropy and anisotropy of magnetic hydrogels are also presented in this study. The isotropic samples were cured without applying a magnetic field (MF), and the anisotropic samples were cured by applying an MF in the direction perpendicular to the thickness of the samples. The effects of the size, content, and inner structures of magnetic particles on the magneto-responsive and swelling properties of magnetic hydrogels were investigated. It was found that the magnetorheological (MR) effect of anisotropic samples was apparently higher than that of isotropic samples, and the hydrogels with CI exhibited a noticeable MR effect than those with Fe<sub>3</sub>O<sub>4</sub>. The storage modulus can be enhanced by increasing the filler content and size, forming an anisotropic structure, and applying an external MF. In addition, the magnetic hydrogels also have a swelling ability that can be tuned by varying the content and size of the particle fillers.Chanchan XuBin LiXiaojie WangMDPI AGarticlemagnetic hydrogelsmagneto-rheologymagnetitecarbonyl ironwater-swellingBiology (General)QH301-705.5ChemistryQD1-999ENInternational Journal of Molecular Sciences, Vol 22, Iss 12342, p 12342 (2021)
institution DOAJ
collection DOAJ
language EN
topic magnetic hydrogels
magneto-rheology
magnetite
carbonyl iron
water-swelling
Biology (General)
QH301-705.5
Chemistry
QD1-999
spellingShingle magnetic hydrogels
magneto-rheology
magnetite
carbonyl iron
water-swelling
Biology (General)
QH301-705.5
Chemistry
QD1-999
Chanchan Xu
Bin Li
Xiaojie Wang
A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles
description This work investigates the mechanical properties, microstructures, and water-swelling behavior of a novel hydrogel filled with magnetic particles. The nanoparticles of magnetite (Fe<sub>3</sub>O<sub>4</sub>) and the micro-particles of carbonyl iron (CI) were selected and filled into a polyacrylamide (PAAM) hydrogel matrix to create two types of magnetic hydrogels. The isotropy and anisotropy of magnetic hydrogels are also presented in this study. The isotropic samples were cured without applying a magnetic field (MF), and the anisotropic samples were cured by applying an MF in the direction perpendicular to the thickness of the samples. The effects of the size, content, and inner structures of magnetic particles on the magneto-responsive and swelling properties of magnetic hydrogels were investigated. It was found that the magnetorheological (MR) effect of anisotropic samples was apparently higher than that of isotropic samples, and the hydrogels with CI exhibited a noticeable MR effect than those with Fe<sub>3</sub>O<sub>4</sub>. The storage modulus can be enhanced by increasing the filler content and size, forming an anisotropic structure, and applying an external MF. In addition, the magnetic hydrogels also have a swelling ability that can be tuned by varying the content and size of the particle fillers.
format article
author Chanchan Xu
Bin Li
Xiaojie Wang
author_facet Chanchan Xu
Bin Li
Xiaojie Wang
author_sort Chanchan Xu
title A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles
title_short A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles
title_full A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles
title_fullStr A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles
title_full_unstemmed A Comparison Study on the Magneto-Responsive Properties and Swelling Behaviors of a Polyacrylamide-Based Hydrogel Incorporating with Magnetic Particles
title_sort comparison study on the magneto-responsive properties and swelling behaviors of a polyacrylamide-based hydrogel incorporating with magnetic particles
publisher MDPI AG
publishDate 2021
url https://doaj.org/article/7cb01f2fad3b45b0935c8447bfd9c732
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