Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR

Abstract Microwave spin resonance behavior of the Fe3O4 surface decorated ZnO nanocomposites (FZNC) has been investigated by ferromagnetic resonance (FMR). Modified hydrothermal method has been adopted to fabricate FZNC samples with Fe3O4 nanoparticles chains were used as seeds in the uniform magnet...

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Autores principales: Saurabh Pathak, Rajni Verma, Sakshi Singhal, Raghav Chaturvedi, Prashant Kumar, Pragati Sharma, R. P. Pant, Xu Wang
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Publicado: Nature Portfolio 2021
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spelling oai:doaj.org-article:7ebe0299b3bf4c0fb9d244eb51da52132021-12-02T14:03:58ZSpin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR10.1038/s41598-021-83394-82045-2322https://doaj.org/article/7ebe0299b3bf4c0fb9d244eb51da52132021-02-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-83394-8https://doaj.org/toc/2045-2322Abstract Microwave spin resonance behavior of the Fe3O4 surface decorated ZnO nanocomposites (FZNC) has been investigated by ferromagnetic resonance (FMR). Modified hydrothermal method has been adopted to fabricate FZNC samples with Fe3O4 nanoparticles chains were used as seeds in the uniform magnetic field to decorate them on the surface of the ZnO nanoparticles in a unique configuration. Spin dynamics investigation confirms the transition of ZnO from diamagnetic to ferromagnetic as the sharp FMR spectra converts to the broad spectra with Fe3O4 nanoparticles incorporation. A single broad FMR spectra confirms that no isolated Fe3+ or Zn2+ ions exist which is also in agreement with XRD confirming suitable composite formation. Further, the increase in Fe3O4 concentration leads to decrease in g-value which is resulting from the internal field enhancement due to magnetic ordering. Also, various spin resonance parameters were calculated for the FZNC which provides a detail information about the magnetic ordering, exchange coupling and anisotropy. Elemental analysis confirms the presence of Fe and Zn simultaneously and transmission electron microscopy (TEM) image show the presence of Fe3O4 on the grain boundaries of ZnO which has been confirmed by taking high-resolution TEM and electron diffraction patterns on both sides of the interface. These unique structural configuration of the FZNC has tremendous potential in various magneto-optoelectronic, spintronics and electro-chemical applications.Saurabh PathakRajni VermaSakshi SinghalRaghav ChaturvediPrashant KumarPragati SharmaR. P. PantXu WangNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-12 (2021)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Saurabh Pathak
Rajni Verma
Sakshi Singhal
Raghav Chaturvedi
Prashant Kumar
Pragati Sharma
R. P. Pant
Xu Wang
Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR
description Abstract Microwave spin resonance behavior of the Fe3O4 surface decorated ZnO nanocomposites (FZNC) has been investigated by ferromagnetic resonance (FMR). Modified hydrothermal method has been adopted to fabricate FZNC samples with Fe3O4 nanoparticles chains were used as seeds in the uniform magnetic field to decorate them on the surface of the ZnO nanoparticles in a unique configuration. Spin dynamics investigation confirms the transition of ZnO from diamagnetic to ferromagnetic as the sharp FMR spectra converts to the broad spectra with Fe3O4 nanoparticles incorporation. A single broad FMR spectra confirms that no isolated Fe3+ or Zn2+ ions exist which is also in agreement with XRD confirming suitable composite formation. Further, the increase in Fe3O4 concentration leads to decrease in g-value which is resulting from the internal field enhancement due to magnetic ordering. Also, various spin resonance parameters were calculated for the FZNC which provides a detail information about the magnetic ordering, exchange coupling and anisotropy. Elemental analysis confirms the presence of Fe and Zn simultaneously and transmission electron microscopy (TEM) image show the presence of Fe3O4 on the grain boundaries of ZnO which has been confirmed by taking high-resolution TEM and electron diffraction patterns on both sides of the interface. These unique structural configuration of the FZNC has tremendous potential in various magneto-optoelectronic, spintronics and electro-chemical applications.
format article
author Saurabh Pathak
Rajni Verma
Sakshi Singhal
Raghav Chaturvedi
Prashant Kumar
Pragati Sharma
R. P. Pant
Xu Wang
author_facet Saurabh Pathak
Rajni Verma
Sakshi Singhal
Raghav Chaturvedi
Prashant Kumar
Pragati Sharma
R. P. Pant
Xu Wang
author_sort Saurabh Pathak
title Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR
title_short Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR
title_full Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR
title_fullStr Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR
title_full_unstemmed Spin dynamics investigations of multifunctional ambient scalable Fe3O4 surface decorated ZnO magnetic nanocomposite using FMR
title_sort spin dynamics investigations of multifunctional ambient scalable fe3o4 surface decorated zno magnetic nanocomposite using fmr
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/7ebe0299b3bf4c0fb9d244eb51da5213
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