Promoting H2O2 production via 2-electron oxygen reduction by coordinating partially oxidized Pd with defect carbon

Electrocatalysts which deliver high selectivity for two-electron oxygen reduction to hydrogen peroxide in acidic media are sought to replace the conventional anthraquinone process. Here, the authors develop partially oxidised palladium clusters on carbon nanotubes with near 100% selectivity.

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Detalles Bibliográficos
Autores principales: Qiaowan Chang, Pu Zhang, Amir Hassan Bagherzadeh Mostaghimi, Xueru Zhao, Steven R. Denny, Ji Hoon Lee, Hongpeng Gao, Ying Zhang, Huolin L. Xin, Samira Siahrostami, Jingguang G. Chen, Zheng Chen
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/7f4014c359204c46b2e2d1576daa6eab
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Descripción
Sumario:Electrocatalysts which deliver high selectivity for two-electron oxygen reduction to hydrogen peroxide in acidic media are sought to replace the conventional anthraquinone process. Here, the authors develop partially oxidised palladium clusters on carbon nanotubes with near 100% selectivity.