Engineering electrocatalytic activity in nanosized perovskite cobaltite through surface spin-state transition

The activity of electrocatalysts exhibits a strong dependence on their electronic structures. Here, the authors manipulate the eg filling of perovskite cobaltite LaCoO3nanoparticles by changing particle size and show improved oxygen evolution activity with increased numbers of surface high-spin coba...

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Autores principales: Shiming Zhou, Xianbing Miao, Xu Zhao, Chao Ma, Yuhao Qiu, Zhenpeng Hu, Jiyin Zhao, Lei Shi, Jie Zeng
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2016
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Acceso en línea:https://doaj.org/article/82763ab7e4d74ba087491b8d769dbef7
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Sumario:The activity of electrocatalysts exhibits a strong dependence on their electronic structures. Here, the authors manipulate the eg filling of perovskite cobaltite LaCoO3nanoparticles by changing particle size and show improved oxygen evolution activity with increased numbers of surface high-spin cobalt ions.