Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%.
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Nature Portfolio
2021
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oai:doaj.org-article:881645c19d0e4a4cb80c0a20183d98062021-12-02T15:26:52ZStable, active CO2 reduction to formate via redox-modulated stabilization of active sites10.1038/s41467-021-25573-92041-1723https://doaj.org/article/881645c19d0e4a4cb80c0a20183d98062021-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-25573-9https://doaj.org/toc/2041-1723Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%.Le LiAdnan OzdenShuyi GuoF. Pelayo Garcı́a de ArquerChuanhao WangMingzhe ZhangJin ZhangHaoyang JiangWei WangHao DongDavid SintonEdward H. SargentMiao ZhongNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021) |
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Science Q Le Li Adnan Ozden Shuyi Guo F. Pelayo Garcı́a de Arquer Chuanhao Wang Mingzhe Zhang Jin Zhang Haoyang Jiang Wei Wang Hao Dong David Sinton Edward H. Sargent Miao Zhong Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites |
description |
Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%. |
format |
article |
author |
Le Li Adnan Ozden Shuyi Guo F. Pelayo Garcı́a de Arquer Chuanhao Wang Mingzhe Zhang Jin Zhang Haoyang Jiang Wei Wang Hao Dong David Sinton Edward H. Sargent Miao Zhong |
author_facet |
Le Li Adnan Ozden Shuyi Guo F. Pelayo Garcı́a de Arquer Chuanhao Wang Mingzhe Zhang Jin Zhang Haoyang Jiang Wei Wang Hao Dong David Sinton Edward H. Sargent Miao Zhong |
author_sort |
Le Li |
title |
Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites |
title_short |
Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites |
title_full |
Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites |
title_fullStr |
Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites |
title_full_unstemmed |
Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites |
title_sort |
stable, active co2 reduction to formate via redox-modulated stabilization of active sites |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/881645c19d0e4a4cb80c0a20183d9806 |
work_keys_str_mv |
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