Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites

Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%.

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Auteurs principaux:	Le Li, Adnan Ozden, Shuyi Guo, F. Pelayo Garcı́a de Arquer, Chuanhao Wang, Mingzhe Zhang, Jin Zhang, Haoyang Jiang, Wei Wang, Hao Dong, David Sinton, Edward H. Sargent, Miao Zhong
Format:	article
Langue:	EN
Publié:	Nature Portfolio 2021
Sujets:	Science Q
Accès en ligne:	https://doaj.org/article/881645c19d0e4a4cb80c0a20183d9806
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spelling	oai:doaj.org-article:881645c19d0e4a4cb80c0a20183d98062021-12-02T15:26:52ZStable, active CO2 reduction to formate via redox-modulated stabilization of active sites10.1038/s41467-021-25573-92041-1723https://doaj.org/article/881645c19d0e4a4cb80c0a20183d98062021-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-25573-9https://doaj.org/toc/2041-1723Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%.Le LiAdnan OzdenShuyi GuoF. Pelayo Garcı́a de ArquerChuanhao WangMingzhe ZhangJin ZhangHaoyang JiangWei WangHao DongDavid SintonEdward H. SargentMiao ZhongNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Le Li Adnan Ozden Shuyi Guo F. Pelayo Garcı́a de Arquer Chuanhao Wang Mingzhe Zhang Jin Zhang Haoyang Jiang Wei Wang Hao Dong David Sinton Edward H. Sargent Miao Zhong Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
description	Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%.
format	article
author	Le Li Adnan Ozden Shuyi Guo F. Pelayo Garcı́a de Arquer Chuanhao Wang Mingzhe Zhang Jin Zhang Haoyang Jiang Wei Wang Hao Dong David Sinton Edward H. Sargent Miao Zhong
author_facet	Le Li Adnan Ozden Shuyi Guo F. Pelayo Garcı́a de Arquer Chuanhao Wang Mingzhe Zhang Jin Zhang Haoyang Jiang Wei Wang Hao Dong David Sinton Edward H. Sargent Miao Zhong
author_sort	Le Li
title	Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
title_short	Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
title_full	Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
title_fullStr	Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
title_full_unstemmed	Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites
title_sort	stable, active co2 reduction to formate via redox-modulated stabilization of active sites
publisher	Nature Portfolio
publishDate	2021
url	https://doaj.org/article/881645c19d0e4a4cb80c0a20183d9806
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Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites

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