The role of anharmonic phonons in under-barrier spin relaxation of single molecule magnets

Single molecule magnets exhibit faster spin relaxation rates than expected from models based on tunnelling through the relaxation barrier. Here, the authors show, using first principles calculations, that anharmonic spin-phonon interactions may explain the under-barrier spin relaxation.

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Auteurs principaux: Alessandro Lunghi, Federico Totti, Roberta Sessoli, Stefano Sanvito
Format: article
Langue:EN
Publié: Nature Portfolio 2017
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Accès en ligne:https://doaj.org/article/88934cc8f6114a3985f864f95c2baaab
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