Local structure and distortions of mixed methane-carbon dioxide hydrates

Natural gas can be collected from hydrate deposits by exchange with CO2, but the ensuing mixed hydrates and the path to a complete exchange are not fully understood. Here, computational analyses of neutron pair distribution functions of CH4, CO2 and mixed CH4-CO2 hydrates at 10 K reveal that the beh...

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Autores principales:	Bernadette R. Cladek, S. Michelle Everett, Marshall T. McDonnell, Matthew G. Tucker, David J. Keffer, Claudia J. Rawn
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2021
Materias:	Chemistry QD1-999
Acceso en línea:	https://doaj.org/article/88cc77b5378e4ebea4dc45835058e95f
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spelling	oai:doaj.org-article:88cc77b5378e4ebea4dc45835058e95f2021-12-02T10:49:07ZLocal structure and distortions of mixed methane-carbon dioxide hydrates10.1038/s42004-020-00441-72399-3669https://doaj.org/article/88cc77b5378e4ebea4dc45835058e95f2021-01-01T00:00:00Zhttps://doi.org/10.1038/s42004-020-00441-7https://doaj.org/toc/2399-3669Natural gas can be collected from hydrate deposits by exchange with CO2, but the ensuing mixed hydrates and the path to a complete exchange are not fully understood. Here, computational analyses of neutron pair distribution functions of CH4, CO2 and mixed CH4-CO2 hydrates at 10 K reveal that the behavior of mixed gas species cannot be interpolated from properties of pure compounds.Bernadette R. CladekS. Michelle EverettMarshall T. McDonnellMatthew G. TuckerDavid J. KefferClaudia J. RawnNature PortfolioarticleChemistryQD1-999ENCommunications Chemistry, Vol 4, Iss 1, Pp 1-7 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Chemistry QD1-999
spellingShingle	Chemistry QD1-999 Bernadette R. Cladek S. Michelle Everett Marshall T. McDonnell Matthew G. Tucker David J. Keffer Claudia J. Rawn Local structure and distortions of mixed methane-carbon dioxide hydrates
description	Natural gas can be collected from hydrate deposits by exchange with CO2, but the ensuing mixed hydrates and the path to a complete exchange are not fully understood. Here, computational analyses of neutron pair distribution functions of CH4, CO2 and mixed CH4-CO2 hydrates at 10 K reveal that the behavior of mixed gas species cannot be interpolated from properties of pure compounds.
format	article
author	Bernadette R. Cladek S. Michelle Everett Marshall T. McDonnell Matthew G. Tucker David J. Keffer Claudia J. Rawn
author_facet	Bernadette R. Cladek S. Michelle Everett Marshall T. McDonnell Matthew G. Tucker David J. Keffer Claudia J. Rawn
author_sort	Bernadette R. Cladek
title	Local structure and distortions of mixed methane-carbon dioxide hydrates
title_short	Local structure and distortions of mixed methane-carbon dioxide hydrates
title_full	Local structure and distortions of mixed methane-carbon dioxide hydrates
title_fullStr	Local structure and distortions of mixed methane-carbon dioxide hydrates
title_full_unstemmed	Local structure and distortions of mixed methane-carbon dioxide hydrates
title_sort	local structure and distortions of mixed methane-carbon dioxide hydrates
publisher	Nature Portfolio
publishDate	2021
url	https://doaj.org/article/88cc77b5378e4ebea4dc45835058e95f
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Local structure and distortions of mixed methane-carbon dioxide hydrates

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