Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout

Abstract Simple, inexpensive and rapid sensing systems are very demanded for a myriad of uses. Intrinsic properties of emerging paper-based analytical devices have demonstrated considerable potential to fulfill such demand. This work reports an easy-to-use, low cost, and disposable paper-based sensi...

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Autores principales: Ruslan Álvarez-Diduk, Jahir Orozco, Arben Merkoçi
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Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/8aae72d88dd0473881fe9915c0edb4bc
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spelling oai:doaj.org-article:8aae72d88dd0473881fe9915c0edb4bc2021-12-02T11:53:07ZPaper strip-embedded graphene quantum dots: a screening device with a smartphone readout10.1038/s41598-017-01134-32045-2322https://doaj.org/article/8aae72d88dd0473881fe9915c0edb4bc2017-04-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-01134-3https://doaj.org/toc/2045-2322Abstract Simple, inexpensive and rapid sensing systems are very demanded for a myriad of uses. Intrinsic properties of emerging paper-based analytical devices have demonstrated considerable potential to fulfill such demand. This work reports an easy-to-use, low cost, and disposable paper-based sensing device for rapid chemical screening with a smartphone readout. The device comprises luminescent graphene quantum dots (GQDs) sensing probes embedded into a nitrocellulose matrix where the resonance energy transfer phenomenon seems to be the sensing mechanism. The GQDs probes were synthesized from citric acid by a pyrolysis procedure, further physisorbed and confined into small wax-traced spots on the nitrocellulose substrate. The GQDs were excited by an UV LED, this, is powered by a smartphone used as both; energy source and imaging capture. The LED was contained within a 3D-printed dark chamber that isolates the paper platform from external light fluctuations leading to highly reproducible data. The cellulose-based device was proven as a promising screening tool for phenols and polyphenols in environmental and food samples, respectively. It opens up new opportunities for simple and fast screening of organic compounds and offers numerous possibilities for versatile applications. It can be especially useful in remote settings where sophisticated instrumentation is not always available.Ruslan Álvarez-DidukJahir OrozcoArben MerkoçiNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Ruslan Álvarez-Diduk
Jahir Orozco
Arben Merkoçi
Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
description Abstract Simple, inexpensive and rapid sensing systems are very demanded for a myriad of uses. Intrinsic properties of emerging paper-based analytical devices have demonstrated considerable potential to fulfill such demand. This work reports an easy-to-use, low cost, and disposable paper-based sensing device for rapid chemical screening with a smartphone readout. The device comprises luminescent graphene quantum dots (GQDs) sensing probes embedded into a nitrocellulose matrix where the resonance energy transfer phenomenon seems to be the sensing mechanism. The GQDs probes were synthesized from citric acid by a pyrolysis procedure, further physisorbed and confined into small wax-traced spots on the nitrocellulose substrate. The GQDs were excited by an UV LED, this, is powered by a smartphone used as both; energy source and imaging capture. The LED was contained within a 3D-printed dark chamber that isolates the paper platform from external light fluctuations leading to highly reproducible data. The cellulose-based device was proven as a promising screening tool for phenols and polyphenols in environmental and food samples, respectively. It opens up new opportunities for simple and fast screening of organic compounds and offers numerous possibilities for versatile applications. It can be especially useful in remote settings where sophisticated instrumentation is not always available.
format article
author Ruslan Álvarez-Diduk
Jahir Orozco
Arben Merkoçi
author_facet Ruslan Álvarez-Diduk
Jahir Orozco
Arben Merkoçi
author_sort Ruslan Álvarez-Diduk
title Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
title_short Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
title_full Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
title_fullStr Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
title_full_unstemmed Paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
title_sort paper strip-embedded graphene quantum dots: a screening device with a smartphone readout
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/8aae72d88dd0473881fe9915c0edb4bc
work_keys_str_mv AT ruslanalvarezdiduk paperstripembeddedgraphenequantumdotsascreeningdevicewithasmartphonereadout
AT jahirorozco paperstripembeddedgraphenequantumdotsascreeningdevicewithasmartphonereadout
AT arbenmerkoci paperstripembeddedgraphenequantumdotsascreeningdevicewithasmartphonereadout
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