Electron-phonon coupling in topological surface states: The role of polar optical modes

Abstract The use of topological edge states for spintronic applications could be severely hampered by limited lifetimes due to intrinsic many-body interactions, in particular electron-phonon coupling. Previous works to determine the intrinsic coupling strength did not provide a coherent answer. Here...

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Autores principales: Rolf Heid, Irina Yu. Sklyadneva, Evgueni V. Chulkov
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/8b0dcf72b79e468da247194c813dfe09
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spelling oai:doaj.org-article:8b0dcf72b79e468da247194c813dfe092021-12-02T12:32:14ZElectron-phonon coupling in topological surface states: The role of polar optical modes10.1038/s41598-017-01128-12045-2322https://doaj.org/article/8b0dcf72b79e468da247194c813dfe092017-04-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-01128-1https://doaj.org/toc/2045-2322Abstract The use of topological edge states for spintronic applications could be severely hampered by limited lifetimes due to intrinsic many-body interactions, in particular electron-phonon coupling. Previous works to determine the intrinsic coupling strength did not provide a coherent answer. Here, the electron-phonon interaction in the metallic surface state of 3D topological insulators is revised within a first principles framework. For the archetypical cases of Bi2Se3 and Bi2Te3, we find an overall weak coupling constant of less than 0.15, but with a characteristic energy dependence. Derived electronic self-energies compare favorably with previous angle-resolved photoemission spectroscopy results. The prevailing coupling is carried by optical modes of polar character, which is weakly screened by the metallic surface state and can be reduced by doping into bulk bands. We do not find any indication of a strong coupling to the A1g mode or the presence of a Kohn anomaly in the surface phonon spectrum. The weak intrinsic electron-phonon coupling guarantees long-lived quasiparticles at elevated temperatures.Rolf HeidIrina Yu. SklyadnevaEvgueni V. ChulkovNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Rolf Heid
Irina Yu. Sklyadneva
Evgueni V. Chulkov
Electron-phonon coupling in topological surface states: The role of polar optical modes
description Abstract The use of topological edge states for spintronic applications could be severely hampered by limited lifetimes due to intrinsic many-body interactions, in particular electron-phonon coupling. Previous works to determine the intrinsic coupling strength did not provide a coherent answer. Here, the electron-phonon interaction in the metallic surface state of 3D topological insulators is revised within a first principles framework. For the archetypical cases of Bi2Se3 and Bi2Te3, we find an overall weak coupling constant of less than 0.15, but with a characteristic energy dependence. Derived electronic self-energies compare favorably with previous angle-resolved photoemission spectroscopy results. The prevailing coupling is carried by optical modes of polar character, which is weakly screened by the metallic surface state and can be reduced by doping into bulk bands. We do not find any indication of a strong coupling to the A1g mode or the presence of a Kohn anomaly in the surface phonon spectrum. The weak intrinsic electron-phonon coupling guarantees long-lived quasiparticles at elevated temperatures.
format article
author Rolf Heid
Irina Yu. Sklyadneva
Evgueni V. Chulkov
author_facet Rolf Heid
Irina Yu. Sklyadneva
Evgueni V. Chulkov
author_sort Rolf Heid
title Electron-phonon coupling in topological surface states: The role of polar optical modes
title_short Electron-phonon coupling in topological surface states: The role of polar optical modes
title_full Electron-phonon coupling in topological surface states: The role of polar optical modes
title_fullStr Electron-phonon coupling in topological surface states: The role of polar optical modes
title_full_unstemmed Electron-phonon coupling in topological surface states: The role of polar optical modes
title_sort electron-phonon coupling in topological surface states: the role of polar optical modes
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/8b0dcf72b79e468da247194c813dfe09
work_keys_str_mv AT rolfheid electronphononcouplingintopologicalsurfacestatestheroleofpolaropticalmodes
AT irinayusklyadneva electronphononcouplingintopologicalsurfacestatestheroleofpolaropticalmodes
AT evguenivchulkov electronphononcouplingintopologicalsurfacestatestheroleofpolaropticalmodes
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