The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars

Sewage treatment processes are a serious environmental threat due to the difficulties involved in its waste management and disposal. Therefore, one developing trend in sewage sludge processing is its thermal treatment, which generates sewage sludge ash that may contain many environmental pollutants,...

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Autores principales: Erick Grünhäuser Soares, João Castro-Gomes, Mateusz Sitarz, Tomasz Zdeb, Izabela Hager
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Publicado: MDPI AG 2021
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spelling oai:doaj.org-article:8e258046d513488c9fbfa57535235f342021-11-25T19:05:17ZThe Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars10.3390/su1322128932071-1050https://doaj.org/article/8e258046d513488c9fbfa57535235f342021-11-01T00:00:00Zhttps://www.mdpi.com/2071-1050/13/22/12893https://doaj.org/toc/2071-1050Sewage treatment processes are a serious environmental threat due to the difficulties involved in its waste management and disposal. Therefore, one developing trend in sewage sludge processing is its thermal treatment, which generates sewage sludge ash that may contain many environmental pollutants, such as heavy metals. Moreover, due to the European Union requirements that not only focus on the waste generation reduction but also on its reuse and final disposal, it is essential to pursue new applications of such resources, such as the waste-based material incorporation into alternative cementitious materials. Thus, this study evaluated the heavy metals leachability of CO<sub>2</sub>-cured mortars incorporating sewage sludge ash as filler. For this purpose, Portland cement, reactive magnesia, and electric arc furnace slag were used to produce three different CO<sub>2</sub>-cured mortars, which were cured though pressurised accelerated carbonation curing for 24h. These mortars presented up to 12.7 MPa as compressive strength and their carbonation was confirmed by TG-DTG and FT-IR analyses. Their leachability of heavy metals met the European requirements for all waste materials, including inert materials, and post-industrial wastewater. Therefore, the immobilisation of heavy metals in this binding technology may be considered an effective method to safely manage sewage sludge ash.Erick Grünhäuser SoaresJoão Castro-GomesMateusz SitarzTomasz ZdebIzabela HagerMDPI AGarticleCO<sub>2</sub>-cured mortarCO<sub>2</sub> adsorptionheavy metal immobilisationleachingsewage sludge ashelectric arc furnace slagEnvironmental effects of industries and plantsTD194-195Renewable energy sourcesTJ807-830Environmental sciencesGE1-350ENSustainability, Vol 13, Iss 12893, p 12893 (2021)
institution DOAJ
collection DOAJ
language EN
topic CO<sub>2</sub>-cured mortar
CO<sub>2</sub> adsorption
heavy metal immobilisation
leaching
sewage sludge ash
electric arc furnace slag
Environmental effects of industries and plants
TD194-195
Renewable energy sources
TJ807-830
Environmental sciences
GE1-350
spellingShingle CO<sub>2</sub>-cured mortar
CO<sub>2</sub> adsorption
heavy metal immobilisation
leaching
sewage sludge ash
electric arc furnace slag
Environmental effects of industries and plants
TD194-195
Renewable energy sources
TJ807-830
Environmental sciences
GE1-350
Erick Grünhäuser Soares
João Castro-Gomes
Mateusz Sitarz
Tomasz Zdeb
Izabela Hager
The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars
description Sewage treatment processes are a serious environmental threat due to the difficulties involved in its waste management and disposal. Therefore, one developing trend in sewage sludge processing is its thermal treatment, which generates sewage sludge ash that may contain many environmental pollutants, such as heavy metals. Moreover, due to the European Union requirements that not only focus on the waste generation reduction but also on its reuse and final disposal, it is essential to pursue new applications of such resources, such as the waste-based material incorporation into alternative cementitious materials. Thus, this study evaluated the heavy metals leachability of CO<sub>2</sub>-cured mortars incorporating sewage sludge ash as filler. For this purpose, Portland cement, reactive magnesia, and electric arc furnace slag were used to produce three different CO<sub>2</sub>-cured mortars, which were cured though pressurised accelerated carbonation curing for 24h. These mortars presented up to 12.7 MPa as compressive strength and their carbonation was confirmed by TG-DTG and FT-IR analyses. Their leachability of heavy metals met the European requirements for all waste materials, including inert materials, and post-industrial wastewater. Therefore, the immobilisation of heavy metals in this binding technology may be considered an effective method to safely manage sewage sludge ash.
format article
author Erick Grünhäuser Soares
João Castro-Gomes
Mateusz Sitarz
Tomasz Zdeb
Izabela Hager
author_facet Erick Grünhäuser Soares
João Castro-Gomes
Mateusz Sitarz
Tomasz Zdeb
Izabela Hager
author_sort Erick Grünhäuser Soares
title The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars
title_short The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars
title_full The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars
title_fullStr The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars
title_full_unstemmed The Immobilisation of Heavy Metals from Sewage Sludge Ash in CO<sub>2</sub>-Cured Mortars
title_sort immobilisation of heavy metals from sewage sludge ash in co<sub>2</sub>-cured mortars
publisher MDPI AG
publishDate 2021
url https://doaj.org/article/8e258046d513488c9fbfa57535235f34
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