Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4
Crystalline porous catalysts with single Cu sites are dedicated to exploring the dependence of CO2 electroreduction selectivity on the coordination environment of catalytic sites. The conductive MOF Cu-DBC with oxygen-coordinated Cu sites shows a high Faradaic efficiency ~80% of CO2-to-CH4.
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Nature Portfolio
2021
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oai:doaj.org-article:8ee2727469ef40118cad5038aa0bf7422021-11-08T11:12:38ZCoordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH410.1038/s41467-021-26724-82041-1723https://doaj.org/article/8ee2727469ef40118cad5038aa0bf7422021-11-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-26724-8https://doaj.org/toc/2041-1723Crystalline porous catalysts with single Cu sites are dedicated to exploring the dependence of CO2 electroreduction selectivity on the coordination environment of catalytic sites. The conductive MOF Cu-DBC with oxygen-coordinated Cu sites shows a high Faradaic efficiency ~80% of CO2-to-CH4.Yu ZhangLong-Zhang DongShan LiXin HuangJia-Nan ChangJian-Hui WangJie ZhouShun-Li LiYa-Qian LanNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021) |
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Science Q Yu Zhang Long-Zhang Dong Shan Li Xin Huang Jia-Nan Chang Jian-Hui Wang Jie Zhou Shun-Li Li Ya-Qian Lan Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4 |
description |
Crystalline porous catalysts with single Cu sites are dedicated to exploring the dependence of CO2 electroreduction selectivity on the coordination environment of catalytic sites. The conductive MOF Cu-DBC with oxygen-coordinated Cu sites shows a high Faradaic efficiency ~80% of CO2-to-CH4. |
format |
article |
author |
Yu Zhang Long-Zhang Dong Shan Li Xin Huang Jia-Nan Chang Jian-Hui Wang Jie Zhou Shun-Li Li Ya-Qian Lan |
author_facet |
Yu Zhang Long-Zhang Dong Shan Li Xin Huang Jia-Nan Chang Jian-Hui Wang Jie Zhou Shun-Li Li Ya-Qian Lan |
author_sort |
Yu Zhang |
title |
Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4 |
title_short |
Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4 |
title_full |
Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4 |
title_fullStr |
Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4 |
title_full_unstemmed |
Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4 |
title_sort |
coordination environment dependent selectivity of single-site-cu enriched crystalline porous catalysts in co2 reduction to ch4 |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/8ee2727469ef40118cad5038aa0bf742 |
work_keys_str_mv |
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_version_ |
1718442355916275712 |