High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
Highly stretched and conductive hydrogels, especially synthetized from natural polymers, are beneficial for highly stretched electronic equipment which is applied in extreme environment. We designed and prepared robust and tough alginate hydrogels (GMA-SA-PAM) using the ingenious strategy of fully i...
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2021
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oai:doaj.org-article:91613c3e92294867909d4eb3ace8ec6e2021-12-05T14:10:47ZHigh strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide1618-722910.1515/epoly-2021-0043https://doaj.org/article/91613c3e92294867909d4eb3ace8ec6e2021-05-01T00:00:00Zhttps://doi.org/10.1515/epoly-2021-0043https://doaj.org/toc/1618-7229Highly stretched and conductive hydrogels, especially synthetized from natural polymers, are beneficial for highly stretched electronic equipment which is applied in extreme environment. We designed and prepared robust and tough alginate hydrogels (GMA-SA-PAM) using the ingenious strategy of fully interpenetrating cross-linking, in which the glycidyl methacrylate (GMA) was used to modify sodium alginate (SA) and then copolymerized with acrylamide (AM) and methylenebisacrylamide (BIS) as cross-linkers. The complete cross-linked structures can averagely dissipate energy and the polymer structures can maintain hydrogels that are three-dimensional to greatly improve the mechanical performance of hydrogels. The GMA-SA-PAM hydrogels display ultra-stretchable (strain up to ∼407% of tensile strain) and highly compressible (∼57% of compression strain) properties. In addition, soaking the GMA-SA-PAM hydrogel in 5 wt% NaCl solution also endows the conductivity of the hydrogel (this hydrogel was named as GSP-Na) with excellent conductive properties (5.26 S m−1). The GSP-Na hydrogel with high stability, durability, as well as wide range extent sensor is also demonstrated by researching the electrochemical signals and showing the potential for applications in wearable and quickly responded electronics.Liu TaoZhang RipengLiu JianzhiZhao LingYu YueqinDe Gruyterarticlehydrogelfully interpenetratingmechanical strengthalginateacrylamidePolymers and polymer manufactureTP1080-1185ENe-Polymers, Vol 21, Iss 1, Pp 391-397 (2021) |
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hydrogel fully interpenetrating mechanical strength alginate acrylamide Polymers and polymer manufacture TP1080-1185 |
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hydrogel fully interpenetrating mechanical strength alginate acrylamide Polymers and polymer manufacture TP1080-1185 Liu Tao Zhang Ripeng Liu Jianzhi Zhao Ling Yu Yueqin High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
description |
Highly stretched and conductive hydrogels, especially synthetized from natural polymers, are beneficial for highly stretched electronic equipment which is applied in extreme environment. We designed and prepared robust and tough alginate hydrogels (GMA-SA-PAM) using the ingenious strategy of fully interpenetrating cross-linking, in which the glycidyl methacrylate (GMA) was used to modify sodium alginate (SA) and then copolymerized with acrylamide (AM) and methylenebisacrylamide (BIS) as cross-linkers. The complete cross-linked structures can averagely dissipate energy and the polymer structures can maintain hydrogels that are three-dimensional to greatly improve the mechanical performance of hydrogels. The GMA-SA-PAM hydrogels display ultra-stretchable (strain up to ∼407% of tensile strain) and highly compressible (∼57% of compression strain) properties. In addition, soaking the GMA-SA-PAM hydrogel in 5 wt% NaCl solution also endows the conductivity of the hydrogel (this hydrogel was named as GSP-Na) with excellent conductive properties (5.26 S m−1). The GSP-Na hydrogel with high stability, durability, as well as wide range extent sensor is also demonstrated by researching the electrochemical signals and showing the potential for applications in wearable and quickly responded electronics. |
format |
article |
author |
Liu Tao Zhang Ripeng Liu Jianzhi Zhao Ling Yu Yueqin |
author_facet |
Liu Tao Zhang Ripeng Liu Jianzhi Zhao Ling Yu Yueqin |
author_sort |
Liu Tao |
title |
High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
title_short |
High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
title_full |
High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
title_fullStr |
High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
title_full_unstemmed |
High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
title_sort |
high strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide |
publisher |
De Gruyter |
publishDate |
2021 |
url |
https://doaj.org/article/91613c3e92294867909d4eb3ace8ec6e |
work_keys_str_mv |
AT liutao highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide AT zhangripeng highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide AT liujianzhi highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide AT zhaoling highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide AT yuyueqin highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide |
_version_ |
1718371736395710464 |