High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide

Highly stretched and conductive hydrogels, especially synthetized from natural polymers, are beneficial for highly stretched electronic equipment which is applied in extreme environment. We designed and prepared robust and tough alginate hydrogels (GMA-SA-PAM) using the ingenious strategy of fully i...

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Autores principales: Liu Tao, Zhang Ripeng, Liu Jianzhi, Zhao Ling, Yu Yueqin
Formato: article
Lenguaje:EN
Publicado: De Gruyter 2021
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Acceso en línea:https://doaj.org/article/91613c3e92294867909d4eb3ace8ec6e
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spelling oai:doaj.org-article:91613c3e92294867909d4eb3ace8ec6e2021-12-05T14:10:47ZHigh strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide1618-722910.1515/epoly-2021-0043https://doaj.org/article/91613c3e92294867909d4eb3ace8ec6e2021-05-01T00:00:00Zhttps://doi.org/10.1515/epoly-2021-0043https://doaj.org/toc/1618-7229Highly stretched and conductive hydrogels, especially synthetized from natural polymers, are beneficial for highly stretched electronic equipment which is applied in extreme environment. We designed and prepared robust and tough alginate hydrogels (GMA-SA-PAM) using the ingenious strategy of fully interpenetrating cross-linking, in which the glycidyl methacrylate (GMA) was used to modify sodium alginate (SA) and then copolymerized with acrylamide (AM) and methylenebisacrylamide (BIS) as cross-linkers. The complete cross-linked structures can averagely dissipate energy and the polymer structures can maintain hydrogels that are three-dimensional to greatly improve the mechanical performance of hydrogels. The GMA-SA-PAM hydrogels display ultra-stretchable (strain up to ∼407% of tensile strain) and highly compressible (∼57% of compression strain) properties. In addition, soaking the GMA-SA-PAM hydrogel in 5 wt% NaCl solution also endows the conductivity of the hydrogel (this hydrogel was named as GSP-Na) with excellent conductive properties (5.26 S m−1). The GSP-Na hydrogel with high stability, durability, as well as wide range extent sensor is also demonstrated by researching the electrochemical signals and showing the potential for applications in wearable and quickly responded electronics.Liu TaoZhang RipengLiu JianzhiZhao LingYu YueqinDe Gruyterarticlehydrogelfully interpenetratingmechanical strengthalginateacrylamidePolymers and polymer manufactureTP1080-1185ENe-Polymers, Vol 21, Iss 1, Pp 391-397 (2021)
institution DOAJ
collection DOAJ
language EN
topic hydrogel
fully interpenetrating
mechanical strength
alginate
acrylamide
Polymers and polymer manufacture
TP1080-1185
spellingShingle hydrogel
fully interpenetrating
mechanical strength
alginate
acrylamide
Polymers and polymer manufacture
TP1080-1185
Liu Tao
Zhang Ripeng
Liu Jianzhi
Zhao Ling
Yu Yueqin
High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
description Highly stretched and conductive hydrogels, especially synthetized from natural polymers, are beneficial for highly stretched electronic equipment which is applied in extreme environment. We designed and prepared robust and tough alginate hydrogels (GMA-SA-PAM) using the ingenious strategy of fully interpenetrating cross-linking, in which the glycidyl methacrylate (GMA) was used to modify sodium alginate (SA) and then copolymerized with acrylamide (AM) and methylenebisacrylamide (BIS) as cross-linkers. The complete cross-linked structures can averagely dissipate energy and the polymer structures can maintain hydrogels that are three-dimensional to greatly improve the mechanical performance of hydrogels. The GMA-SA-PAM hydrogels display ultra-stretchable (strain up to ∼407% of tensile strain) and highly compressible (∼57% of compression strain) properties. In addition, soaking the GMA-SA-PAM hydrogel in 5 wt% NaCl solution also endows the conductivity of the hydrogel (this hydrogel was named as GSP-Na) with excellent conductive properties (5.26 S m−1). The GSP-Na hydrogel with high stability, durability, as well as wide range extent sensor is also demonstrated by researching the electrochemical signals and showing the potential for applications in wearable and quickly responded electronics.
format article
author Liu Tao
Zhang Ripeng
Liu Jianzhi
Zhao Ling
Yu Yueqin
author_facet Liu Tao
Zhang Ripeng
Liu Jianzhi
Zhao Ling
Yu Yueqin
author_sort Liu Tao
title High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
title_short High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
title_full High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
title_fullStr High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
title_full_unstemmed High strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
title_sort high strength and conductive hydrogel with fully interpenetrated structure from alginate and acrylamide
publisher De Gruyter
publishDate 2021
url https://doaj.org/article/91613c3e92294867909d4eb3ace8ec6e
work_keys_str_mv AT liutao highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide
AT zhangripeng highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide
AT liujianzhi highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide
AT zhaoling highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide
AT yuyueqin highstrengthandconductivehydrogelwithfullyinterpenetratedstructurefromalginateandacrylamide
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