A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors

Abstract Low operating voltages have been long desired for thin-film transistors (TFTs). However, it is still challenging to realise 1-V operation by using conventional dielectrics due to their low gate capacitances and low breakdown voltages. Recently, electric double layers (EDLs) have been regard...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Xiaochen Ma, Jiawei Zhang, Wensi Cai, Hanbin Wang, Joshua Wilson, Qingpu Wang, Qian Xin, Aimin Song
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2017
Materias:
R
Q
Acceso en línea:https://doaj.org/article/91d78fb2bad14e64bafe18ead1fa6f75
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
id oai:doaj.org-article:91d78fb2bad14e64bafe18ead1fa6f75
record_format dspace
spelling oai:doaj.org-article:91d78fb2bad14e64bafe18ead1fa6f752021-12-02T15:04:53ZA Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors10.1038/s41598-017-00939-62045-2322https://doaj.org/article/91d78fb2bad14e64bafe18ead1fa6f752017-04-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-00939-6https://doaj.org/toc/2045-2322Abstract Low operating voltages have been long desired for thin-film transistors (TFTs). However, it is still challenging to realise 1-V operation by using conventional dielectrics due to their low gate capacitances and low breakdown voltages. Recently, electric double layers (EDLs) have been regarded as a promising candidate for low-power electronics due to their high capacitance. In this work, we present the first sputtered SiO2 solid-state electrolyte. In order to demonstrate EDL behaviour, a sputtered 200 nm-thick SiO2 electrolyte was incorporated into InGaZnO TFTs as the gate dielectric. The devices exhibited an operating voltage of 1 V, a threshold voltage of 0.06 V, a subthreshold swing of 83 mV dec−1 and an on/off ratio higher than 105. The specific capacitance was 0.45 µF cm−2 at 20 Hz, which is around 26 times higher than the value obtained from thermally oxidised SiO2 films with the same thickness. Analysis of the microstructure and mass density of the sputtered SiO2 films under different deposition conditions indicates that such high capacitance might be attributed to mobile protons donated by atmospheric water. The InGaZnO TFTs with the optimised SiO2 electrolyte also showed good air stability. This work provides a new pathway to the realisation of high-yield low-power electronics.Xiaochen MaJiawei ZhangWensi CaiHanbin WangJoshua WilsonQingpu WangQian XinAimin SongNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-6 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Xiaochen Ma
Jiawei Zhang
Wensi Cai
Hanbin Wang
Joshua Wilson
Qingpu Wang
Qian Xin
Aimin Song
A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors
description Abstract Low operating voltages have been long desired for thin-film transistors (TFTs). However, it is still challenging to realise 1-V operation by using conventional dielectrics due to their low gate capacitances and low breakdown voltages. Recently, electric double layers (EDLs) have been regarded as a promising candidate for low-power electronics due to their high capacitance. In this work, we present the first sputtered SiO2 solid-state electrolyte. In order to demonstrate EDL behaviour, a sputtered 200 nm-thick SiO2 electrolyte was incorporated into InGaZnO TFTs as the gate dielectric. The devices exhibited an operating voltage of 1 V, a threshold voltage of 0.06 V, a subthreshold swing of 83 mV dec−1 and an on/off ratio higher than 105. The specific capacitance was 0.45 µF cm−2 at 20 Hz, which is around 26 times higher than the value obtained from thermally oxidised SiO2 films with the same thickness. Analysis of the microstructure and mass density of the sputtered SiO2 films under different deposition conditions indicates that such high capacitance might be attributed to mobile protons donated by atmospheric water. The InGaZnO TFTs with the optimised SiO2 electrolyte also showed good air stability. This work provides a new pathway to the realisation of high-yield low-power electronics.
format article
author Xiaochen Ma
Jiawei Zhang
Wensi Cai
Hanbin Wang
Joshua Wilson
Qingpu Wang
Qian Xin
Aimin Song
author_facet Xiaochen Ma
Jiawei Zhang
Wensi Cai
Hanbin Wang
Joshua Wilson
Qingpu Wang
Qian Xin
Aimin Song
author_sort Xiaochen Ma
title A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors
title_short A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors
title_full A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors
title_fullStr A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors
title_full_unstemmed A Sputtered Silicon Oxide Electrolyte for High-Performance Thin-Film Transistors
title_sort sputtered silicon oxide electrolyte for high-performance thin-film transistors
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/91d78fb2bad14e64bafe18ead1fa6f75
work_keys_str_mv AT xiaochenma asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT jiaweizhang asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT wensicai asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT hanbinwang asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT joshuawilson asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT qingpuwang asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT qianxin asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT aiminsong asputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT xiaochenma sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT jiaweizhang sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT wensicai sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT hanbinwang sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT joshuawilson sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT qingpuwang sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT qianxin sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
AT aiminsong sputteredsiliconoxideelectrolyteforhighperformancethinfilmtransistors
_version_ 1718389029469159424