Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential

While direct N2 reduction using electrochemistry offers an appealing method to obtain usable nitrogen, materials typically show poor activities and efficiencies. Here, authors demonstrate a single-atom catalyst, iron on N-doped carbon, to have dramatically enhanced N2 reduction efficiencies.

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Autores principales: Mengfan Wang, Sisi Liu, Tao Qian, Jie Liu, Jinqiu Zhou, Haoqing Ji, Jie Xiong, Jun Zhong, Chenglin Yan
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2019
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Acceso en línea:https://doaj.org/article/924f3b6222eb45eab2c1c1ea62603fcf
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spelling oai:doaj.org-article:924f3b6222eb45eab2c1c1ea62603fcf2021-12-02T15:35:03ZOver 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential10.1038/s41467-018-08120-x2041-1723https://doaj.org/article/924f3b6222eb45eab2c1c1ea62603fcf2019-01-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-08120-xhttps://doaj.org/toc/2041-1723While direct N2 reduction using electrochemistry offers an appealing method to obtain usable nitrogen, materials typically show poor activities and efficiencies. Here, authors demonstrate a single-atom catalyst, iron on N-doped carbon, to have dramatically enhanced N2 reduction efficiencies.Mengfan WangSisi LiuTao QianJie LiuJinqiu ZhouHaoqing JiJie XiongJun ZhongChenglin YanNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-8 (2019)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Mengfan Wang
Sisi Liu
Tao Qian
Jie Liu
Jinqiu Zhou
Haoqing Ji
Jie Xiong
Jun Zhong
Chenglin Yan
Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
description While direct N2 reduction using electrochemistry offers an appealing method to obtain usable nitrogen, materials typically show poor activities and efficiencies. Here, authors demonstrate a single-atom catalyst, iron on N-doped carbon, to have dramatically enhanced N2 reduction efficiencies.
format article
author Mengfan Wang
Sisi Liu
Tao Qian
Jie Liu
Jinqiu Zhou
Haoqing Ji
Jie Xiong
Jun Zhong
Chenglin Yan
author_facet Mengfan Wang
Sisi Liu
Tao Qian
Jie Liu
Jinqiu Zhou
Haoqing Ji
Jie Xiong
Jun Zhong
Chenglin Yan
author_sort Mengfan Wang
title Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
title_short Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
title_full Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
title_fullStr Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
title_full_unstemmed Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
title_sort over 56.55% faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
publisher Nature Portfolio
publishDate 2019
url https://doaj.org/article/924f3b6222eb45eab2c1c1ea62603fcf
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