Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential
While direct N2 reduction using electrochemistry offers an appealing method to obtain usable nitrogen, materials typically show poor activities and efficiencies. Here, authors demonstrate a single-atom catalyst, iron on N-doped carbon, to have dramatically enhanced N2 reduction efficiencies.
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Nature Portfolio
2019
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oai:doaj.org-article:924f3b6222eb45eab2c1c1ea62603fcf2021-12-02T15:35:03ZOver 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential10.1038/s41467-018-08120-x2041-1723https://doaj.org/article/924f3b6222eb45eab2c1c1ea62603fcf2019-01-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-08120-xhttps://doaj.org/toc/2041-1723While direct N2 reduction using electrochemistry offers an appealing method to obtain usable nitrogen, materials typically show poor activities and efficiencies. Here, authors demonstrate a single-atom catalyst, iron on N-doped carbon, to have dramatically enhanced N2 reduction efficiencies.Mengfan WangSisi LiuTao QianJie LiuJinqiu ZhouHaoqing JiJie XiongJun ZhongChenglin YanNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-8 (2019) |
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Science Q Mengfan Wang Sisi Liu Tao Qian Jie Liu Jinqiu Zhou Haoqing Ji Jie Xiong Jun Zhong Chenglin Yan Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
description |
While direct N2 reduction using electrochemistry offers an appealing method to obtain usable nitrogen, materials typically show poor activities and efficiencies. Here, authors demonstrate a single-atom catalyst, iron on N-doped carbon, to have dramatically enhanced N2 reduction efficiencies. |
format |
article |
author |
Mengfan Wang Sisi Liu Tao Qian Jie Liu Jinqiu Zhou Haoqing Ji Jie Xiong Jun Zhong Chenglin Yan |
author_facet |
Mengfan Wang Sisi Liu Tao Qian Jie Liu Jinqiu Zhou Haoqing Ji Jie Xiong Jun Zhong Chenglin Yan |
author_sort |
Mengfan Wang |
title |
Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
title_short |
Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
title_full |
Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
title_fullStr |
Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
title_full_unstemmed |
Over 56.55% Faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
title_sort |
over 56.55% faradaic efficiency of ambient ammonia synthesis enabled by positively shifting the reaction potential |
publisher |
Nature Portfolio |
publishDate |
2019 |
url |
https://doaj.org/article/924f3b6222eb45eab2c1c1ea62603fcf |
work_keys_str_mv |
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_version_ |
1718386670549598208 |