Are Shockley-Read-Hall and ABC models valid for lead halide perovskites?

Charge dynamics in perovskite is not well-understood, limited by the knowledge of defect physics and charge recombination mechanism, yet the ABC and SRH models are widely used. Here, the authors introduce advanced PLQY mapping as function of excitation pulse energy and repetition frequency to examin...

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Autores principales: Alexander Kiligaridis, Pavel A. Frantsuzov, Aymen Yangui, Sudipta Seth, Jun Li, Qingzhi An, Yana Vaynzof, Ivan G. Scheblykin
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/93b89be280ce46bca497719699d4e762
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Sumario:Charge dynamics in perovskite is not well-understood, limited by the knowledge of defect physics and charge recombination mechanism, yet the ABC and SRH models are widely used. Here, the authors introduce advanced PLQY mapping as function of excitation pulse energy and repetition frequency to examine the validity of these models.