Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure
Abstract Valleytronics is receiving extensive research efforts. Thus, we investigated the electric field-induced valley polarization in the WSe2/CrSnSe3 heterostructures by varying the stacking order. The heterostructure shows indirect band gaps of 270 and 330 meV in the two most stable structures....
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oai:doaj.org-article:95dd76a31ded4f9d8f46c7821ee792782021-12-02T13:35:39ZElectric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure10.1038/s41699-020-00195-92397-7132https://doaj.org/article/95dd76a31ded4f9d8f46c7821ee792782021-01-01T00:00:00Zhttps://doi.org/10.1038/s41699-020-00195-9https://doaj.org/toc/2397-7132Abstract Valleytronics is receiving extensive research efforts. Thus, we investigated the electric field-induced valley polarization in the WSe2/CrSnSe3 heterostructures by varying the stacking order. The heterostructure shows indirect band gaps of 270 and 330 meV in the two most stable structures. The WSe2/CrSnSe3 heterostructure displays a ferromagnetic ground state with out-of-plane anisotropy (0.02 meV) in one stable stacking (S-1) while a small in-plane anisotropy (−0.01 meV) is found in other stacking (S-2). The Curie temperature is slightly enhanced to 73 K compared to the monolayer CrSnSe3. We have found the valley splitting of 4 meV in S-1 whereas it became 9 meV in the S-2 system. The valley splitting is further enhanced if an electric field is applied from CrSnSe3 to the WSe2 layer whereas it is suppressed in the reversed electric field. Particularly, the S-2 structure shows a giant valley splitting of 67 meV at an electric field of 0.6 V Å−1. We attribute this electric field-dependency to the dipolar effect. Overall, we propose that the WSe2/CrSnSe3 heterostructure can be a potential structure for obtaining a giant valley splitting.Imran KhanBrahim MarfouaJisang HongNature PortfolioarticleMaterials of engineering and construction. Mechanics of materialsTA401-492ChemistryQD1-999ENnpj 2D Materials and Applications, Vol 5, Iss 1, Pp 1-8 (2021) |
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Materials of engineering and construction. Mechanics of materials TA401-492 Chemistry QD1-999 Imran Khan Brahim Marfoua Jisang Hong Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure |
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Abstract Valleytronics is receiving extensive research efforts. Thus, we investigated the electric field-induced valley polarization in the WSe2/CrSnSe3 heterostructures by varying the stacking order. The heterostructure shows indirect band gaps of 270 and 330 meV in the two most stable structures. The WSe2/CrSnSe3 heterostructure displays a ferromagnetic ground state with out-of-plane anisotropy (0.02 meV) in one stable stacking (S-1) while a small in-plane anisotropy (−0.01 meV) is found in other stacking (S-2). The Curie temperature is slightly enhanced to 73 K compared to the monolayer CrSnSe3. We have found the valley splitting of 4 meV in S-1 whereas it became 9 meV in the S-2 system. The valley splitting is further enhanced if an electric field is applied from CrSnSe3 to the WSe2 layer whereas it is suppressed in the reversed electric field. Particularly, the S-2 structure shows a giant valley splitting of 67 meV at an electric field of 0.6 V Å−1. We attribute this electric field-dependency to the dipolar effect. Overall, we propose that the WSe2/CrSnSe3 heterostructure can be a potential structure for obtaining a giant valley splitting. |
format |
article |
author |
Imran Khan Brahim Marfoua Jisang Hong |
author_facet |
Imran Khan Brahim Marfoua Jisang Hong |
author_sort |
Imran Khan |
title |
Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure |
title_short |
Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure |
title_full |
Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure |
title_fullStr |
Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure |
title_full_unstemmed |
Electric field induced giant valley polarization in two dimensional ferromagnetic WSe2/CrSnSe3 heterostructure |
title_sort |
electric field induced giant valley polarization in two dimensional ferromagnetic wse2/crsnse3 heterostructure |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/95dd76a31ded4f9d8f46c7821ee79278 |
work_keys_str_mv |
AT imrankhan electricfieldinducedgiantvalleypolarizationintwodimensionalferromagneticwse2crsnse3heterostructure AT brahimmarfoua electricfieldinducedgiantvalleypolarizationintwodimensionalferromagneticwse2crsnse3heterostructure AT jisanghong electricfieldinducedgiantvalleypolarizationintwodimensionalferromagneticwse2crsnse3heterostructure |
_version_ |
1718392688576823296 |