Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination

Abstract Complete theoretical understanding of the most complex superconductors requires a detailed knowledge of the symmetry of the superconducting energy-gap $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α , for all momenta k on the Fermi surface of every band α. While there are a variety of tec...

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Autores principales: Rahul Sharma, Andreas Kreisel, Miguel Antonio Sulangi, Jakob Böker, Andrey Kostin, Milan P. Allan, H. Eisaki, Anna E. Böhmer, Paul C. Canfield, Ilya Eremin, J. C. Séamus Davis, P. J. Hirschfeld, Peter O. Sprau
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Publicado: Nature Portfolio 2021
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spelling oai:doaj.org-article:97145cbfdfec440a8f2c15b397204a4b2021-12-02T15:59:41ZMulti-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination10.1038/s41535-020-00303-42397-4648https://doaj.org/article/97145cbfdfec440a8f2c15b397204a4b2021-01-01T00:00:00Zhttps://doi.org/10.1038/s41535-020-00303-4https://doaj.org/toc/2397-4648Abstract Complete theoretical understanding of the most complex superconductors requires a detailed knowledge of the symmetry of the superconducting energy-gap $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α , for all momenta k on the Fermi surface of every band α. While there are a variety of techniques for determining $$|{\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha |$$ ∣ Δ k α ∣ , no general method existed to measure the signed values of $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α . Recently, however, a technique based on phase-resolved visualization of superconducting quasiparticle interference (QPI) patterns, centered on a single non-magnetic impurity atom, was introduced. In principle, energy-resolved and phase-resolved Fourier analysis of these images identifies wavevectors connecting all k-space regions where $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α has the same or opposite sign. But use of a single isolated impurity atom, from whose precise location the spatial phase of the scattering interference pattern must be measured, is technically difficult. Here we introduce a generalization of this approach for use with multiple impurity atoms, and demonstrate its validity by comparing the $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α it generates to the $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α determined from single-atom scattering in FeSe where s± energy-gap symmetry is established. Finally, to exemplify utility, we use the multi-atom technique on LiFeAs and find scattering interference between the hole-like and electron-like pockets as predicted for $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α of opposite sign.Rahul SharmaAndreas KreiselMiguel Antonio SulangiJakob BökerAndrey KostinMilan P. AllanH. EisakiAnna E. BöhmerPaul C. CanfieldIlya EreminJ. C. Séamus DavisP. J. HirschfeldPeter O. SprauNature PortfolioarticleMaterials of engineering and construction. Mechanics of materialsTA401-492Atomic physics. Constitution and properties of matterQC170-197ENnpj Quantum Materials, Vol 6, Iss 1, Pp 1-7 (2021)
institution DOAJ
collection DOAJ
language EN
topic Materials of engineering and construction. Mechanics of materials
TA401-492
Atomic physics. Constitution and properties of matter
QC170-197
spellingShingle Materials of engineering and construction. Mechanics of materials
TA401-492
Atomic physics. Constitution and properties of matter
QC170-197
Rahul Sharma
Andreas Kreisel
Miguel Antonio Sulangi
Jakob Böker
Andrey Kostin
Milan P. Allan
H. Eisaki
Anna E. Böhmer
Paul C. Canfield
Ilya Eremin
J. C. Séamus Davis
P. J. Hirschfeld
Peter O. Sprau
Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
description Abstract Complete theoretical understanding of the most complex superconductors requires a detailed knowledge of the symmetry of the superconducting energy-gap $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α , for all momenta k on the Fermi surface of every band α. While there are a variety of techniques for determining $$|{\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha |$$ ∣ Δ k α ∣ , no general method existed to measure the signed values of $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α . Recently, however, a technique based on phase-resolved visualization of superconducting quasiparticle interference (QPI) patterns, centered on a single non-magnetic impurity atom, was introduced. In principle, energy-resolved and phase-resolved Fourier analysis of these images identifies wavevectors connecting all k-space regions where $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α has the same or opposite sign. But use of a single isolated impurity atom, from whose precise location the spatial phase of the scattering interference pattern must be measured, is technically difficult. Here we introduce a generalization of this approach for use with multiple impurity atoms, and demonstrate its validity by comparing the $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α it generates to the $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α determined from single-atom scattering in FeSe where s± energy-gap symmetry is established. Finally, to exemplify utility, we use the multi-atom technique on LiFeAs and find scattering interference between the hole-like and electron-like pockets as predicted for $${\mathrm{{\Delta}}}_{\mathbf{k}}^\alpha$$ Δ k α of opposite sign.
format article
author Rahul Sharma
Andreas Kreisel
Miguel Antonio Sulangi
Jakob Böker
Andrey Kostin
Milan P. Allan
H. Eisaki
Anna E. Böhmer
Paul C. Canfield
Ilya Eremin
J. C. Séamus Davis
P. J. Hirschfeld
Peter O. Sprau
author_facet Rahul Sharma
Andreas Kreisel
Miguel Antonio Sulangi
Jakob Böker
Andrey Kostin
Milan P. Allan
H. Eisaki
Anna E. Böhmer
Paul C. Canfield
Ilya Eremin
J. C. Séamus Davis
P. J. Hirschfeld
Peter O. Sprau
author_sort Rahul Sharma
title Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
title_short Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
title_full Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
title_fullStr Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
title_full_unstemmed Multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
title_sort multi-atom quasiparticle scattering interference for superconductor energy-gap symmetry determination
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/97145cbfdfec440a8f2c15b397204a4b
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