High Temporal and Spectral Resolution of Stimulated X-Ray Raman Signals with Stochastic Free-Electron-Laser Pulses

The chaotic nature of x-ray free-electron-laser pulses is a major bottleneck that has limited the joint temporal and spectral resolution of spectroscopic measurements. We show how to use the stochastic x-ray field statistics to overcome this difficulty through correlation signals averaged over indep...

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Bibliographic Details
Main Authors: Stefano M. Cavaletto, Daniel Keefer, Shaul Mukamel
Format: article
Language:EN
Published: American Physical Society 2021
Subjects:
Online Access:https://doaj.org/article/97d112dddfc34b9dbd932ac2bd63262a
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