Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer

The undesirable geological release of methane at remote locations can be lessened through an efficient methane conversion process. Here, the authors report selective ambient functionalization of methane by a vanadium (V)-oxo electrocatalyst with a low activation energy and a high turnover frequency.

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Autores principales: Jiao Deng, Sheng-Chih Lin, Jack Fuller, Jesus A. Iñiguez, Danlei Xiang, Di Yang, Gary Chan, Hao Ming Chen, Anastassia N. Alexandrova, Chong Liu
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/9906f58da3e1440997cb02f9bb2326bf
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spelling oai:doaj.org-article:9906f58da3e1440997cb02f9bb2326bf2021-12-02T16:18:02ZAmbient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer10.1038/s41467-020-17494-w2041-1723https://doaj.org/article/9906f58da3e1440997cb02f9bb2326bf2020-07-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-17494-whttps://doaj.org/toc/2041-1723The undesirable geological release of methane at remote locations can be lessened through an efficient methane conversion process. Here, the authors report selective ambient functionalization of methane by a vanadium (V)-oxo electrocatalyst with a low activation energy and a high turnover frequency.Jiao DengSheng-Chih LinJack FullerJesus A. IñiguezDanlei XiangDi YangGary ChanHao Ming ChenAnastassia N. AlexandrovaChong LiuNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-10 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Jiao Deng
Sheng-Chih Lin
Jack Fuller
Jesus A. Iñiguez
Danlei Xiang
Di Yang
Gary Chan
Hao Ming Chen
Anastassia N. Alexandrova
Chong Liu
Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer
description The undesirable geological release of methane at remote locations can be lessened through an efficient methane conversion process. Here, the authors report selective ambient functionalization of methane by a vanadium (V)-oxo electrocatalyst with a low activation energy and a high turnover frequency.
format article
author Jiao Deng
Sheng-Chih Lin
Jack Fuller
Jesus A. Iñiguez
Danlei Xiang
Di Yang
Gary Chan
Hao Ming Chen
Anastassia N. Alexandrova
Chong Liu
author_facet Jiao Deng
Sheng-Chih Lin
Jack Fuller
Jesus A. Iñiguez
Danlei Xiang
Di Yang
Gary Chan
Hao Ming Chen
Anastassia N. Alexandrova
Chong Liu
author_sort Jiao Deng
title Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer
title_short Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer
title_full Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer
title_fullStr Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer
title_full_unstemmed Ambient methane functionalization initiated by electrochemical oxidation of a vanadium (V)-oxo dimer
title_sort ambient methane functionalization initiated by electrochemical oxidation of a vanadium (v)-oxo dimer
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/9906f58da3e1440997cb02f9bb2326bf
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AT garychan ambientmethanefunctionalizationinitiatedbyelectrochemicaloxidationofavanadiumvoxodimer
AT haomingchen ambientmethanefunctionalizationinitiatedbyelectrochemicaloxidationofavanadiumvoxodimer
AT anastassianalexandrova ambientmethanefunctionalizationinitiatedbyelectrochemicaloxidationofavanadiumvoxodimer
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