Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation

Atomically dispersed metal-N-C are efficient active site for benzene oxidation but the roles of N and C atoms are still unclear. Here the authors report a highly-active single-atom Fe-based benzene oxidation catalyst and provide deep insights into the structure-activity relationship at atomic level.

Guardado en:
Detalles Bibliográficos
Autores principales: Yuan Pan, Yinjuan Chen, Konglin Wu, Zheng Chen, Shoujie Liu, Xing Cao, Weng-Chon Cheong, Tao Meng, Jun Luo, Lirong Zheng, Chenguang Liu, Dingsheng Wang, Qing Peng, Jun Li, Chen Chen
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2019
Materias:
Q
Acceso en línea:https://doaj.org/article/9a0ddaf1313b4074a195c15a8857f4c3
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
Descripción
Sumario:Atomically dispersed metal-N-C are efficient active site for benzene oxidation but the roles of N and C atoms are still unclear. Here the authors report a highly-active single-atom Fe-based benzene oxidation catalyst and provide deep insights into the structure-activity relationship at atomic level.