Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation
Atomically dispersed metal-N-C are efficient active site for benzene oxidation but the roles of N and C atoms are still unclear. Here the authors report a highly-active single-atom Fe-based benzene oxidation catalyst and provide deep insights into the structure-activity relationship at atomic level.
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Nature Portfolio
2019
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oai:doaj.org-article:9a0ddaf1313b4074a195c15a8857f4c32021-12-02T17:02:08ZRegulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation10.1038/s41467-019-12362-82041-1723https://doaj.org/article/9a0ddaf1313b4074a195c15a8857f4c32019-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-12362-8https://doaj.org/toc/2041-1723Atomically dispersed metal-N-C are efficient active site for benzene oxidation but the roles of N and C atoms are still unclear. Here the authors report a highly-active single-atom Fe-based benzene oxidation catalyst and provide deep insights into the structure-activity relationship at atomic level.Yuan PanYinjuan ChenKonglin WuZheng ChenShoujie LiuXing CaoWeng-Chon CheongTao MengJun LuoLirong ZhengChenguang LiuDingsheng WangQing PengJun LiChen ChenNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-11 (2019) |
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EN |
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Science Q Yuan Pan Yinjuan Chen Konglin Wu Zheng Chen Shoujie Liu Xing Cao Weng-Chon Cheong Tao Meng Jun Luo Lirong Zheng Chenguang Liu Dingsheng Wang Qing Peng Jun Li Chen Chen Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation |
description |
Atomically dispersed metal-N-C are efficient active site for benzene oxidation but the roles of N and C atoms are still unclear. Here the authors report a highly-active single-atom Fe-based benzene oxidation catalyst and provide deep insights into the structure-activity relationship at atomic level. |
format |
article |
author |
Yuan Pan Yinjuan Chen Konglin Wu Zheng Chen Shoujie Liu Xing Cao Weng-Chon Cheong Tao Meng Jun Luo Lirong Zheng Chenguang Liu Dingsheng Wang Qing Peng Jun Li Chen Chen |
author_facet |
Yuan Pan Yinjuan Chen Konglin Wu Zheng Chen Shoujie Liu Xing Cao Weng-Chon Cheong Tao Meng Jun Luo Lirong Zheng Chenguang Liu Dingsheng Wang Qing Peng Jun Li Chen Chen |
author_sort |
Yuan Pan |
title |
Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation |
title_short |
Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation |
title_full |
Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation |
title_fullStr |
Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation |
title_full_unstemmed |
Regulating the coordination structure of single-atom Fe-N x C y catalytic sites for benzene oxidation |
title_sort |
regulating the coordination structure of single-atom fe-n x c y catalytic sites for benzene oxidation |
publisher |
Nature Portfolio |
publishDate |
2019 |
url |
https://doaj.org/article/9a0ddaf1313b4074a195c15a8857f4c3 |
work_keys_str_mv |
AT yuanpan regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT yinjuanchen regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT konglinwu regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT zhengchen regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT shoujieliu regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT xingcao regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT wengchoncheong regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT taomeng regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT junluo regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT lirongzheng regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT chenguangliu regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT dingshengwang regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT qingpeng regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT junli regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation AT chenchen regulatingthecoordinationstructureofsingleatomfenxcycatalyticsitesforbenzeneoxidation |
_version_ |
1718381984783269888 |